School of Geography and Tourism, Zhengzhou Normal University, Zhengzhou, People's Republic of China.
School of Water Conservancy, North China University of Water Resources and Electric Power, Zhengzhou, People's Republic of China.
Environ Technol. 2024 Jan;45(3):495-507. doi: 10.1080/09593330.2022.2114015. Epub 2022 Aug 25.
In large river basins, the nitrogen (N) cycle is largely regulated by complicated interactions between human and natural elements. Nevertheless, the origins, fate and driving forces of reactive nitrogen (Nr) flows in the basins are still not clear. An estimation model of N flux was established for evaluating the Nr flow and its environmental effects in the Yellow River Basin of Henan Province (HYRB) by means of material flow analysis. Total N input and output of HYRB were calculated at 4090.9 and 3948.8 Gg N yr, causing 142.0 Gg yr of N stored in the basin. Industry, cropland and residential activities, respectively occupied for 42.2%, 23.2% and 12.3% of the whole input, as well as 43.6%, 25.1% and 12.3% of the whole output, which were central to HYRB's N cycle. Anthropogenic activities regulated above 95.0% of total inputs, and 49.5% of N outputs was emitted into the air and 4.5% into hydrosphere. High N input, energy intensive, imperfect sewage disposal facilities and low N utilization efficiency were the main reasons of contaminate. How to effectively regulate the input of high-strength N pollutant associated with insufficient N cycling and Nr elimination is the main issue in the Yellow River Basin. In present research also put forward corresponding control measures according to the evaluation of N flow and Nr release of HYRB. The research can supply science foundation for coordinating the human-environment relationship in large basins, and also has important reference significance for the formulation of Nr emission reduction strategies.
在大型流域中,氮(N)循环主要受人为和自然因素之间复杂的相互作用调控。然而,流域中活性氮(Nr)流的来源、归宿和驱动力仍不清楚。本研究通过物质流分析,建立氮通量估算模型,评估河南省黄河流域(HYRB)的 Nr 流及其环境效应。计算得出 HYRB 的总氮输入和输出分别为 4090.9 和 3948.8 Gg N yr,导致流域内储存了 142.0 Gg yr 的 N。工业、农田和居民活动分别占总输入的 42.2%、23.2%和 12.3%,也分别占总输出的 43.6%、25.1%和 12.3%,是 HYRB 氮循环的核心。人为活动调控着超过 95.0%的总输入,49.5%的 N 输出排放到大气中,4.5%排放到水圈中。高氮投入、能源密集型、不完善的污水处理设施和低氮利用效率是造成污染的主要原因。如何有效调控与氮循环不足和 Nr 去除相关的高强度氮污染物的输入,是黄河流域面临的主要问题。本研究还根据 HYRB 的氮流和 Nr 释放评估提出了相应的控制措施。本研究可为协调大流域的人-环境关系提供科学依据,对制定 Nr 减排策略也具有重要的参考意义。