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高效自修复近红外钙钛矿发光二极管的制备方案。

Protocol for efficient and self-healing near-infrared perovskite light-emitting diodes.

机构信息

Macao Institute of Materials Science and Engineering, Macau University of Science and Technology, Macau 999078, P. R. China.

Department of Physics, Chemistry and Biology (IFM), Linköping University, Linköping, Sweden.

出版信息

STAR Protoc. 2022 Aug 18;3(3):101631. doi: 10.1016/j.xpro.2022.101631. eCollection 2022 Sep 16.

DOI:10.1016/j.xpro.2022.101631
PMID:36035792
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC9405535/
Abstract

Preparation of highly efficient and stable perovskite light-emitting diodes (PeLEDs) with reproducible device performance is challenging. This protocol describes steps for fabrication of high-performance and self-healing PeLEDs. These include instructions for synthesis of charge-transporting zinc oxide (ZnO) nanocrystals, step-by-step device fabrication, and control over self-healing of the degraded devices. For complete details on the use and execution of this protocol, please refer to Teng et al. (2021).

摘要

制备高效稳定且器件性能可重现的钙钛矿发光二极管（PeLED）极具挑战性。本方案描述了制备高性能自修复 PeLED 的步骤。其中包括载流子传输氧化锌（ZnO）纳米晶体的合成说明、分步器件制备以及对退化器件的自修复控制。如需了解本方案使用和实施的详细信息，请参考 Teng 等人（2021 年）。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e83/9405535/1b862684740c/gr9.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e83/9405535/b099dcc5efce/fx1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e83/9405535/aafc261573c0/gr2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e83/9405535/e720e9be0c46/gr1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e83/9405535/33c3c6456664/gr4.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e83/9405535/a6394db33308/gr3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e83/9405535/de859a688bf0/gr5.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e83/9405535/581bd5ef898a/gr6.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e83/9405535/c329917239c1/gr7.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e83/9405535/e23629cb4ae7/gr8.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e83/9405535/1b862684740c/gr9.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e83/9405535/b099dcc5efce/fx1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e83/9405535/aafc261573c0/gr2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e83/9405535/e720e9be0c46/gr1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e83/9405535/33c3c6456664/gr4.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e83/9405535/a6394db33308/gr3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e83/9405535/de859a688bf0/gr5.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e83/9405535/581bd5ef898a/gr6.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e83/9405535/c329917239c1/gr7.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e83/9405535/e23629cb4ae7/gr8.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e83/9405535/1b862684740c/gr9.jpg

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本文引用的文献

1
Revealing a Zinc Oxide/Perovskite Luminescence Quenching Mechanism Targeting Low-Roll-off Light-Emitting Diodes.揭示一种针对低滚降发光二极管的氧化锌/钙钛矿发光猝灭机制。
J Phys Chem Lett. 2022 Apr 7;13(13):3121-3129. doi: 10.1021/acs.jpclett.2c00564. Epub 2022 Mar 31.
2
Manipulating crystallization dynamics through chelating molecules for bright perovskite emitters.通过螯合分子调控结晶动力学以制备明亮的钙钛矿发光体。
Nat Commun. 2021 Aug 10;12(1):4831. doi: 10.1038/s41467-021-25092-7.
3
Impact of Amine Additives on Perovskite Precursor Aging: A Case Study of Light-Emitting Diodes.
胺添加剂对钙钛矿前驱体老化的影响：以发光二极管为例
J Phys Chem Lett. 2021 Jul 1;12(25):5836-5843. doi: 10.1021/acs.jpclett.1c01349. Epub 2021 Jun 17.
4
Phenylalkylammonium passivation enables perovskite light emitting diodes with record high-radiance operational lifetime: the chain length matters.苯基烷基铵钝化使钙钛矿发光二极管具有创纪录的高辐射工作寿命：链长很重要。
Nat Commun. 2021 Jan 28;12(1):644. doi: 10.1038/s41467-021-20970-6.
5
Transparent near-infrared perovskite light-emitting diodes.透明近红外钙钛矿发光二极管
Nat Commun. 2020 Aug 24;11(1):4213. doi: 10.1038/s41467-020-18110-7.
6
Edge stabilization in reduced-dimensional perovskites.低维钙钛矿中的边缘稳定化
Nat Commun. 2020 Jan 10;11(1):170. doi: 10.1038/s41467-019-13944-2.
7
Perovskite light-emitting diodes based on spontaneously formed submicrometre-scale structures.基于自发形成的亚微米级结构的钙钛矿发光二极管。
Nature. 2018 Oct;562(7726):249-253. doi: 10.1038/s41586-018-0576-2. Epub 2018 Oct 10.