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用于能量收集的环保型果胶聚合物薄膜摩擦纳米发电机

Eco-friendly pectin polymer film-based triboelectric nanogenerator for energy scavenging.

作者信息

Patnam Harishkumarreddy, Graham Sontyana Adonijah, Manchi Punnarao, Vasant Paranjape Mandar, Yu Jae Su

机构信息

Department of Electronics and Information Convergence Engineering, Institute for Wearable Convergence Electronics, Kyung Hee University, 1732 Deogyeong-daero, Giheung-gu, Yongin-Si, Gyeonggi-do 17104, Republic of Korea.

出版信息

Nanoscale. 2022 Sep 22;14(36):13236-13247. doi: 10.1039/d1nr07157b.

Abstract

Inspired by the desire to solve the energy-related issues in remote sensing applications, internet of things, wireless autonomous devices, and self-powered portable electronic devices, triboelectric nanogenerators (TENGs) have been highly promoted. However, for use in the specified applications, especially in wearable and biomedical devices, environmental-friendly materials are required. Herein, an eco-friendly pectin polymer is used as a positive triboelectric material to fabricate a TENG with excellent output performance. Working in conjunction with a polyimide, the polyimide and microarchitected pectin (MA@pectin) polymer film-based TENG (PP-TENG) generated open circuit voltage (), short circuit current (), and charge density () of ∼300 V, 14 μA, and 70 μC cm, respectively, exhibiting remarkable enhancement compared to the TENG based on polyimide/pristine pectin polymer (, , and of 170 V, 7.6 μA, and 47 μC cm, respectively) under similar operating conditions. The output performance of the PP-TENG is particularly reliant on the pectin concentration, indicating an optimum concentration of 9 wt%. The improved performance of the PP-TENG was systematically analyzed and explained in terms of pectin concentration, dielectric constant, and surface roughness. Furthermore, the PP-TENG can power portable electronic devices and light-emitting diodes to prove the capability of the TENG in practical applications. The fabricated PP-TENG is anticipated to be a sustainable energy harvester a low-cost and facile approach.

摘要

受解决遥感应用、物联网、无线自主设备和自供电便携式电子设备中与能源相关问题的愿望启发,摩擦纳米发电机(TENG)得到了大力推广。然而,对于特定应用,特别是可穿戴和生物医学设备,需要环保材料。在此,一种环保的果胶聚合物被用作正摩擦电材料来制造具有优异输出性能的TENG。与聚酰亚胺配合使用时,基于聚酰亚胺和微结构果胶(MA@果胶)聚合物薄膜的TENG(PP-TENG)产生的开路电压()、短路电流()和电荷密度()分别约为300 V、14 μA和70 μC/cm²,与在类似操作条件下基于聚酰亚胺/原始果胶聚合物的TENG(开路电压、短路电流和电荷密度分别为170 V、7.6 μA和47 μC/cm²)相比,有显著提高。PP-TENG的输出性能特别依赖于果胶浓度,表明最佳浓度为9 wt%。从果胶浓度、介电常数和表面粗糙度方面对PP-TENG的性能改进进行了系统分析和解释。此外,PP-TENG可以为便携式电子设备和发光二极管供电,以证明TENG在实际应用中的能力。所制造的PP-TENG有望成为一种低成本且简便的可持续能量收集器。

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