Addor Yao S, Baumgardner Darrel, Hughes Dagen, Newman Nicholas, Jandarov Roman, Reponen Tiina
University of Cincinnati, Department of the Environmental and Public Health Sciences, Cincinnati, OH, USA.
Droplet Measurement Technologies LLC., 2400 Trade Centre Avenue, Longmont, CO 80503, USA.
Environ Sci Process Impacts. 2022 Oct 19;24(10):1790-1804. doi: 10.1039/d2em00177b.
We assessed and compared indoor and outdoor residential aerosol particles in a third-floor apartment from August through September 2020. The measurements were conducted using a direct-reading ultraviolet light-induced fluorescence (UV-LIF) wideband integrated bioaerosol spectrometer (WIBS). It measures individual particle light scattering and fluorescence from which particle properties can be derived. The number concentrations of total aerosol particles (TAP) and total fluorescent aerosol particles (TFAP) were significantly higher indoors. Daily and hourly TFAP mean concentrations followed the same trends as the TAP, both indoors and outdoors. The daily mean rank of the TFAP fraction (TFAP/TAP) was significantly higher indoors (23%) than outdoors (19%). Particles representing bacteria dominated indoors while particles representing fungi and pollen dominated outdoors. The mean volume-weighted median diameters for TFAP were 1.67 μm indoors and 2.09 μm outdoors. Higher TFAP fraction indoors was likely due to occupants' activities that generated or resuspended particles. This study contributes to understanding the characteristics of residential aerosol particles in situations when occupants spend most of their time indoors. Based on our findings, a large portion of all indoor aerosol particles could be biological (15-20%) and of respirable particle size (≥95%). Using a novel direct reading UV-LIF-based sensor can help quickly assess aerosol exposures relevant to human health.
2020年8月至9月,我们对一套三楼公寓的室内和室外住宅气溶胶颗粒进行了评估和比较。测量使用的是直读式紫外光诱导荧光(UV-LIF)宽带综合生物气溶胶光谱仪(WIBS)。它测量单个颗粒的光散射和荧光,由此可以得出颗粒的特性。室内总气溶胶颗粒(TAP)和总荧光气溶胶颗粒(TFAP)的数量浓度显著更高。室内和室外,TFAP的每日和每小时平均浓度与TAP的趋势相同。TFAP分数(TFAP/TAP)的每日平均排名在室内(23%)显著高于室外(19%)。代表细菌的颗粒在室内占主导,而代表真菌和花粉的颗粒在室外占主导。TFAP的平均体积加权中值直径在室内为1.67μm,在室外为2.09μm。室内TFAP分数较高可能是由于居住者的活动产生或重新悬浮了颗粒。这项研究有助于了解居住者大部分时间待在室内时住宅气溶胶颗粒的特征。根据我们的研究结果,所有室内气溶胶颗粒中有很大一部分可能是生物性的(15%-20%)且具有可吸入粒径(≥95%)。使用基于UV-LIF的新型直读式传感器有助于快速评估与人类健康相关的气溶胶暴露情况。