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阳极结构对含油污泥沉积微生物燃料电池性能的影响

Effect of the Anode Structure on the Performance of Oily Sludge Sediment Microbial Fuel Cells.

作者信息

Guo Haiying, Ren Wen, Huang Chunfeng, Yang Qi, Tang Shanfa, Geng Xiaoheng, Jia Xinlei

机构信息

Department of Chemical Engineering and Safety Engineering, Binzhou University, Binzhou, Shandong 256600, China.

School of Water Resource and Environment, China University of Geosciences (Beijing), Beijing 100083, China.

出版信息

ACS Omega. 2022 Aug 15;7(34):29959-29966. doi: 10.1021/acsomega.2c02976. eCollection 2022 Aug 30.

Abstract

The anode is considered to be a key factor to improve the single-chamber bioelectrochemical system's efficiency to degrade oily sludge in sediment while generating electricity. There are few studies on the effect of the anode structure on the performance of oily sludge MFCs systematically. In this paper, an oily sludge bioelectrical system was constructed using carbon felt and carbon plate as anode materials, adjusting the anode material arrangement as transverse and longitudinal, and using different anode materials from single to sextuple anodes. The results of this study showed that the rate of degradation of oily sludge was greater with carbon felt (17.04%) than with the carbon plate (13.11%), with transverse (23.61%) than with the longitudinal (19.82%) arrangement of anodes, and with sextuple anodes (33.72%) than with a single anode (25.26%) in the sediment microbial fuel cells (SMFCs). A similar trend was observed when the voltage, power density, and electromotive force (EMF) of SMFCs were estimated between the carbon felt and carbon plate, transverse and longitudinal arrangements, single and sextuple anodes. It is concluded that the proper adjustment of anode arrangements, using carbon felt as an anode material, and increasing the number of anodes to six may accelerate the rate of degradation of oily sludge in oily sludge sediment microbial fuel cells (SMFCs). Furthermore, the electricity generation performance was also improved.

摘要

阳极被认为是提高单室生物电化学系统在沉积物中降解含油污泥效率并同时发电的关键因素。关于阳极结构对含油污泥微生物燃料电池性能的影响,系统的研究较少。本文以碳毡和碳板作为阳极材料构建了含油污泥生物电系统,将阳极材料排列调整为横向和纵向,并使用从单阳极到六重阳极的不同阳极材料。本研究结果表明,在沉积物微生物燃料电池(SMFC)中,碳毡作为阳极时含油污泥的降解率(17.04%)高于碳板(13.11%),阳极横向排列(23.61%)时高于纵向排列(19.82%),六重阳极(33.72%)时高于单阳极(25.26%)。当估算SMFC在碳毡和碳板、横向和纵向排列、单阳极和六重阳极之间的电压、功率密度和电动势(EMF)时,观察到类似趋势。得出的结论是,在含油污泥沉积物微生物燃料电池(SMFC)中,适当调整阳极排列,使用碳毡作为阳极材料,并将阳极数量增加到六个,可能会加速含油污泥的降解速率。此外,发电性能也得到了改善。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/52b5/9434775/126c7e9ca4ab/ao2c02976_0002.jpg

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