Lerner E, Bouchbinder E
Institute for Theoretical Physics, University of Amsterdam, Science Park 904, 1098 XH Amsterdam, Netherlands.
Chemical and Biological Physics Department, Weizmann Institute of Science, Rehovot 7610001, Israel.
Phys Rev Lett. 2022 Aug 26;129(9):095501. doi: 10.1103/PhysRevLett.129.095501.
Structural glasses formed by quenching a melt are known to host a population of low-energy quasilocalized (nonphononic) excitations whose frequencies ω follow a universal ∼ω^{4} distribution as ω→0, independently of the glass formation history, the interparticle interaction potential, or spatial dimension. Here, we show that the universal quartic law of nonphononic excitations also holds in disordered crystals featuring finite long-range order, which is absent in their glassy counterparts. We thus establish that the degree of universality of the quartic law extends beyond structural glasses quenched from a melt. We further find that disordered crystals, whose level of disorder can be continuously controlled, host many more quasilocalized excitations than expected based on their degree of mechanical disorder-quantified by the relative fluctuations of the shear modulus-as compared to structural glasses featuring a similar degree of mechanical disorder. Our results are related to glasslike anomalies experimentally observed in disordered crystals. More broadly, they constitute an important step toward tracing the essential ingredients necessary for the emergence of universal nonphononic excitations in disordered solids.
通过淬冷熔体形成的结构玻璃已知含有一群低能准局域化(非声子)激发,其频率ω在ω→0时遵循通用的~ω⁴分布,与玻璃形成历史、粒子间相互作用势或空间维度无关。在此,我们表明非声子激发的通用四次方定律在具有有限长程有序的无序晶体中也成立,而其玻璃态对应物中不存在这种长程有序。因此,我们确定四次方定律的普遍性程度超出了从熔体淬冷的结构玻璃。我们还进一步发现,与具有相似机械无序程度的结构玻璃相比,其无序程度可连续控制的无序晶体所拥有的准局域化激发比基于其机械无序程度(由剪切模量的相对波动量化)预期的要多得多。我们的结果与在无序晶体中实验观察到的类玻璃异常现象有关。更广泛地说,它们是朝着追踪无序固体中出现通用非声子激发所需的基本要素迈出的重要一步。