State Key Laboratory of Loess and Quaternary Geology, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an 710061, China; National Observation and Research Station of Regional Ecological Environment Change and Comprehensive Management in the Guanzhong Plain, Shaanxi, China.
School of Human Settlements and Civil Engineering, Xi'an Jiaotong University, Xi'an 710049, China.
Sci Total Environ. 2022 Dec 20;853:158597. doi: 10.1016/j.scitotenv.2022.158597. Epub 2022 Sep 8.
Atmospheric humidity has been shown to promote haze formation, but it remains unclear why the air is humid during heavy haze days in winter. Here we combine water vapor isotope measurements with WRF-Chem simulations to elucidate increasing humidity with aggravation of haze during wintertime in urban Beijing. The vapor isotopic analysis in Beijing shows that the combustion-derived water (CDW) constitutes 11.0± 6.2 % of the atmospheric moisture and its fraction in total moisture increases with aggravation of haze. Modeling results reveal that, in addition to the water vapor transported from south or east to Beijing with occurrence of haze, CDW has a considerable impact on the increasing humidity when haze becomes heavy or severe. Aerosol-radiation interactions generally decrease the water vapor content and only increase humidity with occurrence of severe haze with hourly PM concentrations exceeding 250μg m. Although CDW is insignificant in the global atmospheric vapor budget, it could play an important role in modifying the local weather during haze days.
大气湿度已被证明会促进霾的形成,但目前仍不清楚为什么在冬季重霾天气中空气会潮湿。在这里,我们结合水汽同位素测量和 WRF-Chem 模拟,阐明了冬季北京城区霾加重时湿度的增加。北京的水汽同位素分析表明,燃烧产生的水(CDW)占大气水汽的 11.0±6.2%,其在总水汽中的比例随着霾的加重而增加。模拟结果表明,除了在出现霾时从南方或东方输送到北京的水汽外,当霾变得严重或严重时,CDW 对湿度的增加也有相当大的影响。气溶胶-辐射相互作用通常会降低水汽含量,只有在出现严重霾且每小时 PM2.5 浓度超过 250μg m 时,才会增加湿度。尽管 CDW 在全球大气水汽预算中微不足道,但它在霾天气期间改变当地天气方面可能发挥重要作用。