Dipartimento di Fisica, Università degli Studi di Bari and INFN, Sezione di Bari, via Amendola 173, Bari, 70126, Italy.
Centre Européen de Calcul Atomique et Moléculaire (CECAM), Ecole Polytechnique Fédérale de Lausanne (EPFL), Batochimie, Avenue Forel 2, 1015, Lausanne, Switzerland.
Eur Phys J E Soft Matter. 2022 Sep 13;45(9):75. doi: 10.1140/epje/s10189-022-00230-1.
We study numerically the role of hydrodynamics in the liquid-hexatic transition of active colloids at intermediate activity, where motility induced phase separation (MIPS) does not occur. We show that in the case of active Brownian particles (ABP), the critical density of the transition decreases upon increasing the particle's mass, enhancing ordering, while self-propulsion has the opposite effect in the activity regime considered. Active hydrodynamic particles (AHP), instead, undergo the liquid-hexatic transition at higher values of packing fraction [Formula: see text] than the corresponding ABP, suggesting that hydrodynamics have the net effect of disordering the system. At increasing densities, close to the hexatic-liquid transition, we found in the case of AHP the appearance of self-sustained organized motion with clusters of particles moving coherently.
我们通过数值研究了在中间活性下,活性胶体的液体-六方相转变中流体动力学的作用,在这个活性范围内不会发生由迁移诱导相分离(MIPS)引起的相分离。结果表明,对于活性布朗粒子(ABP),当颗粒质量增加时,转变的临界密度降低,从而增强了有序性,而在考虑的活性范围内,自推进则产生相反的效果。相反,活性流体粒子(AHP)在高于相应 ABP 的填充分数[Formula: see text]时经历液体-六方相转变,这表明流体动力学具有使系统无序的净效应。在接近六方-液体转变的较高密度下,我们发现 AHP 中出现了具有自持续组织运动的颗粒团簇的相干运动。