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外场活性乳液中的软通道形成和对称破缺。

Soft channel formation and symmetry breaking in exotic active emulsions.

机构信息

Dipartimento di Fisica, Università degli Srudi di Bari and INFN, Sezione di Bari, Via Amendola 173, 70126, Bari, Italy.

IAC - CNR, Via Amendola, 122/D, 70126, Bari, Italy.

出版信息

Sci Rep. 2020 Sep 28;10(1):15936. doi: 10.1038/s41598-020-72742-9.

Abstract

We use computer simulations to study the morphology and rheological properties of a bidimensional emulsion resulting from a mixture of a passive isotropic fluid and an active contractile polar gel, in the presence of a surfactant that favours the emulsification of the two phases. By varying the intensity of the contractile activity and of an externally imposed shear flow, we find three possible morphologies. For low shear rates, a simple lamellar state is obtained. For intermediate activity and shear rate, an asymmetric state emerges, which is characterized by shear and concentration banding at the polar/isotropic interface. A further increment in the active forcing leads to the self-assembly of a soft channel where an isotropic fluid flows between two layers of active material. We characterize the stability of this state by performing a dynamical test varying the intensity of the active forcing and shear rate. Finally, we address the rheological properties of the system by measuring the effective shear viscosity, finding that this increases as active forcing is increased-so that the fluid thickens with activity.

摘要

我们使用计算机模拟来研究二维乳液的形态和流变性质,这种乳液是由被动各向同性流体和主动收缩性极性凝胶混合而成,其中存在一种表面活性剂,有利于两相的乳化。通过改变收缩活性和外部施加的剪切流的强度,我们发现了三种可能的形态。对于低剪切速率,获得简单的层状状态。对于中等活性和剪切速率,出现不对称状态,其特征在于在极性/各向同性界面处的剪切和浓度带状。进一步增加主动力导致软通道的自组装,其中各向同性流体在两层活性材料之间流动。我们通过执行一个动态测试来改变主动力和剪切速率的强度来表征这种状态的稳定性。最后,我们通过测量有效剪切粘度来研究系统的流变性质,发现随着主动力的增加,有效剪切粘度增加,因此随着活性的增加,流体变厚。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b82b/7522284/49c14f6efadb/41598_2020_72742_Fig1_HTML.jpg

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