Liu Zhixin, Ling Qian, Cai Yawen, Xu Linfeng, Su Jiahao, Yu Kuai, Wu Xinyi, Xu Jiayi, Hu Baowei, Wang Xiangke
School of Life Science, Shaoxing University Huancheng West Road 508 Shaoxing 312000 China
Nanoscale Adv. 2022 Jan 20;4(5):1246-1262. doi: 10.1039/d1na00843a. eCollection 2022 Mar 1.
With the fast development of industry, large amounts of organic and inorganic pollutants are inevitably released into the natural environment, which results in the pollution of the environment and are thereby dangerous to human health. The efficient elimination of these pollutants is crucial to environment protection and human health. The high sorption capacity of carbon-based materials and high photocatalytic ability of carbon-based composites result in the application of carbon-based materials in environmental pollution cleanup. In this review article, we summarized recent studies on the synthesis of carbon-based materials, and their application in the sorption of organic and inorganic pollutants, the photocatalytic degradation of organic pollutants, and the photocatalytic reduction-solidification of heavy metal ions. The sorption method is useful to remove pollutants from aqueous solutions. The sorption-photocatalytic degradation of organic pollutants is applicable, especially at low concentrations, whereas the catalytic reduction of metal ions is the best method for the immobilization of high valent metal ions under complicated conditions. The interaction mechanism is discussed using advanced spectroscopy analysis and theoretical calculations, and at the end the challenges in the future are described.
随着工业的快速发展,大量有机和无机污染物不可避免地排放到自然环境中,这导致了环境污染,进而对人类健康构成威胁。有效消除这些污染物对于环境保护和人类健康至关重要。碳基材料的高吸附能力和碳基复合材料的高光催化能力使得碳基材料在环境污染清理中得到应用。在这篇综述文章中,我们总结了碳基材料合成的最新研究,以及它们在有机和无机污染物吸附、有机污染物光催化降解和重金属离子光催化还原固化方面的应用。吸附法有助于从水溶液中去除污染物。有机污染物的吸附-光催化降解是适用的,特别是在低浓度情况下,而金属离子的催化还原是在复杂条件下固定高价金属离子的最佳方法。利用先进的光谱分析和理论计算讨论了相互作用机制,最后描述了未来面临的挑战。