Department of Chemistry and Biochemistry, School of Mathematics and Natural Sciences, University of Southern Mississippi, Hattiesburg, Mississippi39406, United States.
Department of Computer Science, Virginia Commonwealth University, Richmond, Virginia23220, United States.
Biochemistry. 2022 Oct 18;61(20):2206-2220. doi: 10.1021/acs.biochem.2c00495. Epub 2022 Sep 29.
A major hallmark of Alzheimer's disease (AD) is the accumulation of extracellular aggregates of amyloid-β (Aβ). Structural polymorphism observed among Aβ fibrils in AD brains seem to correlate with the clinical subtypes suggesting a link between fibril polymorphism and pathology. Since fibrils emerge from a templated growth of low-molecular-weight oligomers, understanding the factors affecting oligomer generation is important. Membrane lipids are key factors to influence early stages of Aβ aggregation and oligomer generation, which cause membrane disruption. We have previously demonstrated that conformationally discrete Aβ oligomers can be generated by modulating the charge, composition, and chain length of lipids and surfactants. Here, we extend our studies into liposomal models by investigating Aβ oligomerization on large unilamellar vesicles (LUVs) of total brain extracts (TBE), reconstituted lipid rafts (LRs), or 1,2-dimyristoyl-sn-glycero-3-phosphocholine (DMPC). Varying the vesicle composition by specifically increasing the amount of GM1 gangliosides as a constituent, we found that only GM1-enriched liposomes induce the formation of toxic, low-molecular-weight oligomers. Furthermore, we found that the aggregation on liposome surface and membrane disruption are highly cooperative and sensitive to membrane surface characteristics. Numerical simulations confirm such a cooperativity and reveal that GM1-enriched liposomes form twice as many pores as those formed in the absence GM1. Overall, this study uncovers mechanisms of cooperativity between oligomerization and membrane disruption under controlled lipid compositional bias, and refocuses the significance of the early stages of Aβ aggregation in polymorphism, propagation, and toxicity in AD.
阿尔茨海默病(AD)的一个主要标志是细胞外淀粉样β(Aβ)聚集物的积累。AD 大脑中观察到的 Aβ 纤维中的结构多态性似乎与临床亚型相关,表明纤维多态性与病理学之间存在联系。由于纤维从低分子量寡聚物的模板生长中出现,因此了解影响寡聚物生成的因素很重要。膜脂质是影响 Aβ聚集和寡聚物生成的关键因素,这会导致膜破裂。我们之前已经证明,通过调节电荷、组成和链长,可以生成构象离散的 Aβ 寡聚物脂质和表面活性剂。在这里,我们通过研究总脑提取物(TBE)、重建的脂筏(LR)或 1,2-二肉豆蔻酰-sn-甘油-3-磷酸胆碱(DMPC)的大单室囊泡(LUV)上的 Aβ 寡聚化,将我们的研究扩展到脂质体模型中。通过特别增加 GM1 神经节苷脂作为组成部分来改变囊泡组成,我们发现只有富含 GM1 的脂质体才能诱导形成有毒的低分子量寡聚物。此外,我们发现,在脂质体表面上的聚集和膜破裂具有高度的协同作用,并且对膜表面特性非常敏感。数值模拟证实了这种协同作用,并表明富含 GM1 的脂质体形成的孔是 GM1 不存在时形成的孔的两倍。总的来说,这项研究揭示了在受控脂质组成偏倚下,寡聚化和膜破坏之间的协同作用机制,并重新关注了 Aβ 聚集在 AD 中的多态性、传播和毒性的早期阶段的重要性。