Dubé Kimberlee, Randel William, Bourassa Adam, Degenstein Doug
Institute of Space and Atmospheric Studies University of Saskatchewan Saskatoon SK Canada.
National Center for Atmospheric Research Boulder CO USA.
Geophys Res Lett. 2022 Sep 28;49(18):e2022GL099848. doi: 10.1029/2022GL099848. Epub 2022 Sep 14.
Deep convection within the Asian summer monsoon (ASM) transports surface level air into the upper troposphere-lower stratosphere (UTLS). This work aims to understand the distribution of NO, NO, and NO in the UTLS ASM anticyclone from satellite measurements. Observations of NO from the Optical Spectrograph and InfraRed Imager System, the Atmospheric Chemistry Experiment - Fourier Transform Spectrometer (ACE-FTS), and the Stratospheric Aerosol and Gas Experiment III on the International Space Station are considered. The PRATMO photochemical box model is used to quantify the NO photochemistry, and to derive the NO concentration using OSIRIS NO and O observations. The satellite data show a relative minimum in NO over the ASM in the summer months, while the corresponding NO and NO anomalies are elevated, mainly due to low O and cold temperatures within the ASM. The observations within the ASM show reasonable agreement to simulations from the Whole Atmosphere Community Climate Model.
亚洲夏季风(ASM)中的深对流将地表空气输送到对流层上部-平流层下部(UTLS)。这项工作旨在通过卫星测量了解UTLS ASM反气旋中一氧化氮(NO)、二氧化氮(NO₂)和一氧化二氮(N₂O)的分布情况。我们考虑了来自光学光谱仪和红外成像系统、大气化学实验-傅里叶变换光谱仪(ACE-FTS)以及国际空间站上的平流层气溶胶和气体实验III对NO的观测数据。PRATMO光化学箱模型用于量化NO光化学,并利用OSIRIS对NO和O的观测数据推导NO浓度。卫星数据显示,在夏季月份,ASM上空的NO相对较低,而相应的NO₂和N₂O异常升高,这主要是由于ASM内部O含量低和温度寒冷所致。ASM内的观测结果与全球大气社区气候模型的模拟结果显示出合理的一致性。