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多共振模式耦合在手性超表面中实现了强烈的圆二色性响应。

Multiple resonant modes coupling enabled strong CD response in a chiral metasurface.

作者信息

Zong Shu, Zeng Dongwen, Liu Guiqiang, Wang Yan, Liu Zhengqi, Chen Jing

出版信息

Opt Express. 2022 Oct 24;30(22):40470-40481. doi: 10.1364/OE.475060.

Abstract

The chiral structures with strong circular dichroism (CD) response and narrow linewidth are desirable in chiral sensing, circularly-polarized light detection, and polarization imaging. Here, we theoretically proposed a hybrid chiral metasurface for differential absorption of circularly polarized light. Based on the multiple resonant modes coupling effect in a two-dimensional dielectric slab, it is realizable then to achieve a nearly perfect absorption for right circularly polarized light and simultaneously reflects 90% of left circularly polarized light, suggesting the generation of strong CD of 0.886 within a narrowly spectral linewidth of 4.53 nm. The multipole analysis reveals that the electric dipole, the magnetic dipole, and the electric quadrupole make dominant contributions to chiral absorption and the high CD response in this metsurface. The excitation of guided mode resonance enhances the ability of this metasurface to absorb electric field. Moreover, the optical chirality response can be further manipulated through the geometry features. These findings pave a powerful way to realize the narrowing and strong CD platform for single-band and multiband chirality behaviors.

摘要

具有强圆二色性(CD)响应和窄线宽的手性结构在手性传感、圆偏振光检测和偏振成像中具有重要应用价值。在此,我们从理论上提出了一种用于圆偏振光差分吸收的混合手性超表面。基于二维介质平板中的多重共振模式耦合效应,可实现对右旋圆偏振光近乎完美的吸收,同时反射90%的左旋圆偏振光,这表明在4.53 nm的窄光谱线宽内产生了0.886的强CD。多极分析表明,电偶极子、磁偶极子和电四极子对该超表面的手性吸收和高CD响应起主要作用。导模共振的激发增强了该超表面吸收电场的能力。此外,光学手性响应可通过几何特征进一步调控。这些发现为实现单波段和多波段手性行为的窄化和强CD平台开辟了一条有力途径。

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