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在河川生态系统中不同水流条件下微塑料颗粒的分散和传输。

Dispersal and transport of microplastic particles under different flow conditions in riverine ecosystem.

机构信息

Key Laboratory for Environment and Disaster Monitoring and Evaluation of Hubei, Innovation Academy for Precision Measurement Science and Technology, Chinese Academy of Sciences, Wuhan 430077, China; Department of Biological and Agricultural Engineering & Zachry Department of Civil Engineering, Texas A&M University, College Station, TX 77843-2117, USA.

Key Laboratory for Environment and Disaster Monitoring and Evaluation of Hubei, Innovation Academy for Precision Measurement Science and Technology, Chinese Academy of Sciences, Wuhan 430077, China.

出版信息

J Hazard Mater. 2023 Jan 15;442:130033. doi: 10.1016/j.jhazmat.2022.130033. Epub 2022 Sep 20.

Abstract

Microplastic (MP) pollution is a global issue owing to its potential threats to ecosystems and human health. MP pollution in river ecosystems is widely investigated, but the transport process under different hydrological conditions remain unclear. In this study, an approach of particle tracking in conjunction with hydrodynamic modeling was developed to investigate the dispersal and transport processes of microplastic particles in riverine ecosystem. The concentration and dispersal pattern of polyamide (PA), polyethylene (PE), polypropylene (PP), polystyrene (PS), and polyethylene terephthalate (PET) particles under base flow and flood events with recurrence intervals of 10-year, 20-year and 50-year were identified. Results indicated that rainfall intensity had a significant impact on the microplastic transport in rivers. Higher suspension concentration and lower sedimented concentration were observed in high flow periods, and the sedimented concentration showed a slow increasing trend in the flood recession stage. High water velocity facilitated the microplastic particles to be migrated for a longer distance, and high water flow was conducive to transport more microplastics from source points. Besides, microplastic particles with high density had worse mobility in water and more prone to deposition. PET were likely to be transported for a relatively shorter distance, while PP had higher mobility and took less time to reach the same simulation point. This study put forward an effective approach to understand the transport of MPs in the river. The results obtained are useful to identify pollution hotspots and track pollution paths.

摘要

微塑料(MP)污染是一个全球性问题,因为它可能对生态系统和人类健康造成威胁。河流生态系统中的 MP 污染已得到广泛研究,但不同水文条件下的传输过程仍不清楚。在这项研究中,开发了一种结合水动力模型的粒子跟踪方法,以研究河流生态系统中微塑料颗粒的分散和传输过程。确定了在重现期为 10 年、20 年和 50 年的基流和洪水事件下,聚酰胺(PA)、聚乙烯(PE)、聚丙烯(PP)、聚苯乙烯(PS)和聚对苯二甲酸乙二醇酯(PET)颗粒的浓度和分散模式。结果表明,降雨强度对河流中的微塑料传输有重大影响。在高流量期,悬浮浓度较高,沉降浓度较低,而在洪水退水阶段,沉降浓度呈缓慢增加趋势。高水流速度有利于微塑料颗粒迁移更长的距离,高水流有利于从源点输送更多的微塑料。此外,密度较高的微塑料颗粒在水中的迁移能力较差,更容易沉积。PET 可能会被输送到相对较短的距离,而 PP 具有更高的迁移能力,到达相同模拟点所需的时间更少。本研究提出了一种有效方法来了解 MPs 在河流中的传输。所得结果有助于识别污染热点并跟踪污染路径。

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