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基于 7 年连续观测的中国清洁空气政策后气溶胶垂直特征的变化及其驱动因素。

Variations and drivers of aerosol vertical characterization after clean air policy in China based on 7-years consecutive observations.

机构信息

State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry (LAPC), Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China; University of Chinese Academy of Sciences, Beijing 100049, China.

State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry (LAPC), Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China.

出版信息

J Environ Sci (China). 2023 Mar;125:499-512. doi: 10.1016/j.jes.2022.02.036. Epub 2022 Mar 7.

Abstract

Understanding the aerosol vertical characterization is of great importance to both climate and atmospheric environment. This study investigated the variations of aerosol profiles over eight regions of interest in China after clean air policy (2013-2019) and discussed the drivers of the vertical aerosol structure, using observations from active satellite measurements (CALIPSO). From the annual variation, the amplitude of extinction coefficient profiles showed a decreasing trend with fluctuations, and the maximum was 0.21 km in Beijing-Tianjin-Hebei (JJJ). For regions suffered from air pollution, the variation was greatest below 0.45 km, while it was between 1-1.5 km for Sichuan Basin. The correlation coefficient between the relative humidity (RH) and the extinction coefficient indicated that the increase of RH inhibited the decrease of the extinction coefficient in the Yangtze River Delta. In most regions, the main aerosol subtypes were polluted dust and polluted continental, but they were coarser in JJJ and North West. The frequency of concurrency of dust and polluted dust aerosols decreased in JJJ, but polluted continental aerosols occurred more frequently. Further, the aerosol extinction coefficient profiles under different pollution conditions showed that it changed most during heavy pollution periods in JJJ, especially in 2017, with a significant aerosol loading between ∼700 and 1200 m. The atmospheric reanalysis data revealed that the weak convergence at low level and the divergence at high level supported the upward transport of aerosols in 2017. Overall, the differences in divergence allocation, RH, and wind filed were the main meteorological drivers.

摘要

了解气溶胶的垂直特性对气候和大气环境都非常重要。本研究利用主动卫星测量(CALIPSO)观测结果,调查了中国 8 个重点地区在清洁空气政策(2013-2019 年)后的气溶胶廓线变化,并讨论了垂直气溶胶结构的驱动因素。从年际变化来看,消光系数廓线的振幅呈波动下降趋势,在北京-天津-河北(JJJ)地区最大为 0.21km。对于受空气污染影响的地区,变化最大的是低于 0.45km 的区域,而四川盆地则在 1-1.5km 之间。相对湿度(RH)与消光系数的相关系数表明,RH 的增加抑制了长三角地区消光系数的下降。在大多数地区,主要的气溶胶亚型是污染尘和污染大陆性,但在 JJJ 和西北,它们更粗。在 JJJ 地区,尘和污染尘气溶胶同时出现的频率降低,但污染大陆性气溶胶更频繁。此外,不同污染条件下的气溶胶消光系数廓线表明,2017 年 JJJ 污染较重期间变化最大,气溶胶负荷在 700-1200m 之间显著增加。大气再分析数据表明,低水平的弱辐合和高水平的辐散支持了 2017 年气溶胶的向上输送。总体而言,辐散分配、RH 和风速场的差异是主要的气象驱动因素。

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