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台风通过调节再悬浮泥沙的多重分形粒径来引发河口重金属风险。

Typhoon triggers estuarine heavy metal risk by regulating the multifractal grainsize of resuspended sediment.

机构信息

Key Laboratory of Integrated Regulation and Resource Development on Shallow Lake of Ministry of Education, College of Environment, Hohai University, Nanjing 210098, China; College of Environment, Hohai University, Nanjing 210098, China.

Key Laboratory of Integrated Regulation and Resource Development on Shallow Lake of Ministry of Education, College of Environment, Hohai University, Nanjing 210098, China; College of Environment, Hohai University, Nanjing 210098, China.

出版信息

Sci Total Environ. 2023 Feb 20;860:160510. doi: 10.1016/j.scitotenv.2022.160510. Epub 2022 Nov 28.

Abstract

The turbulent boundary layer generated by wind in the estuarine surface water serves as a main factor affecting the distribution of suspended particulate matter (SPM) and suspended sediment concentration (SSC). In this study, representative typhoon-induced variation of surface fine SPM (<63 μm) was simulated in the Yangtze River Estuary (YRE) under two time scenarios. Each scenario contained four grainsize SPM fractions named Fraction 1 (<8 μm), Fraction 2 (8-16 μm), Fraction 3 (16-32 μm), Fraction 4 (32-63 μm). The typhoon-induced resuspended multifractal SSC quantification (TRMSQ) based on the relationship between SPM grainsize and heavy metal adsorption capacity was proposed to assess the variation in the resuspended threat of heavy metal to 6 key estuarine protected objects (three reservoirs & three national reserves) between Scenarios 1 and 2. The results presented that Fraction 3 exhibited the maximum increment in SSC resuspension mass and longest regression time from typhoon. Combined with TRMSQ, chromium (Cr) was calculated to be the riskiest typhoon-induced factor. The integrated resuspended risk of heavy metals for each protected object tends to increase from the northwest of Chongming Island (1.2) towards the maximum turbidity zone (>9) downstream, with an estuary-wide mean of 3.3.

摘要

河口表水中风产生的紊流边界层是影响悬浮颗粒物(SPM)和悬浮泥沙浓度(SSC)分布的主要因素。本研究在两个时间场景下,模拟了长江河口(YRE)由代表性台风引起的表面细 SPM(<63μm)的变化。每个场景包含四个 SPM 粒级命名为 Fraction 1(<8μm)、Fraction 2(8-16μm)、Fraction 3(16-32μm)、Fraction 4(32-63μm)。基于 SPM 粒级与重金属吸附能力之间的关系,提出了台风诱发的再悬浮多分散 SSC 定量(TRMSQ),以评估场景 1 和 2 之间 6 个关键河口保护区(3 个水库和 3 个国家级保护区)的重金属再悬浮威胁变化。结果表明,Fraction 3 的 SSC 再悬浮质量增量最大,从台风到回归的时间最长。结合 TRMSQ,计算出铬(Cr)是最危险的台风诱发因素。每个保护区的重金属再悬浮风险综合值从崇明岛西北部(1.2)向最大浑浊带(>9)下游方向逐渐增加,河口平均为 3.3。

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