Han Jiaxin, Tang Xiangyu, Yin Zhiming, Wang Kan, Fu Yong, Wang Beiyu, Chen Yanbo, Zhang Chi, Jin Cheng
Opt Express. 2022 Dec 19;30(26):47942-47956. doi: 10.1364/OE.479226.
Extreme-ultraviolet pulses of attosecond duration carrying orbital angular momentum (OAM) can be produced by spectrally filtering vortex high harmonics generated in a gas medium. Here we reveal that fractional high harmonics (FHHs) with non-integer OAM generated by a short duration Laguerre-Gaussian laser beam are origins for the change of helical attosecond pulse train (APT) with azimuthal angle. We show that these harmonics have gap and minimum structures in the annular intensity profile and discontinue phase distribution along azimuthal angle. And each FHH can be expressed as a superposition of OAM modes with integer topological charges. Features of FHH can be identified by coherently combining selected OAM modes. We also uncover that these features are formed after FHH is propagated in gas medium and in vacuum. We finally demonstrate that the generation of FHHs and the dependence of helical APTs on azimuthal angle are changed by varying the macroscopic condition.
通过对气体介质中产生的涡旋高次谐波进行光谱滤波,可以产生携带轨道角动量(OAM)的阿秒持续时间的极紫外脉冲。在此我们揭示,由短持续时间的拉盖尔 - 高斯激光束产生的具有非整数OAM的分数高次谐波(FHH)是螺旋阿秒脉冲序列(APT)随方位角变化的起源。我们表明,这些谐波在环形强度分布中具有能隙和最小值结构,并且沿方位角的相位分布是间断的。并且每个FHH都可以表示为具有整数拓扑电荷的OAM模式的叠加。FHH的特征可以通过相干地组合选定的OAM模式来识别。我们还发现,这些特征是在FHH在气体介质和真空中传播之后形成的。我们最终证明,通过改变宏观条件,可以改变FHH的产生以及螺旋APT对方位角的依赖性。