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利用携带非零轨道角动量的贝塞尔-高斯光束控制高次谐波的环形空间分布。

Control of the annular spatial profile of high harmonics using a Bessel-Gaussian beam carrying the nonzero orbital angular momentum.

作者信息

Han Jiaxin, Tang Xiangyu, Fu Yong, Wang Beiyu, Yin Zhiming, Jin Cheng

出版信息

Opt Express. 2023 Dec 18;31(26):43732-43747. doi: 10.1364/OE.502772.

DOI:10.1364/OE.502772
PMID:38178463
Abstract

We propose to generate vortex high harmonics in the extreme ultraviolet (XUV) with a controllable spatial profile by using a Bessel-Gaussian (BG) beam carrying a nonzero orbital angular momentum (OAM). Such BG beam has quite a different intensity profile at the focus compared to the generally used BG beam without carrying the OAM. We show that the BG beam is capable of generating single-ring structured high harmonics, which is quite different from an Laguerre-Gaussian (LG) beam with a similar intensity distribution at the laser focus. We reveal that favorable phase-matching conditions can be achieved off-axis and away from the laser focus because a single-atom intrinsic phase due to the short electron trajectory can be well compensated by a geometric phase of the BG beam. We thus give a general rule that vortex high harmonics with a single annular profile can be efficiently generated when a gas medium is located at 1.5z to 2.0z before or after the laser focus of the BG beam, here z is a reduced length. We also show the validity of this rule when the BG beam carries a higher OAM. This work is expected to be useful for synthesizing attosecond vortex pulses.

摘要

我们提议通过使用携带非零轨道角动量(OAM)的贝塞尔 - 高斯(BG)光束,在极紫外(XUV)波段产生具有可控空间分布的涡旋高次谐波。与通常使用的不携带OAM的BG光束相比,这种携带OAM的BG光束在焦点处具有截然不同的强度分布。我们表明,该BG光束能够产生单环结构的高次谐波,这与在激光焦点处具有相似强度分布的拉盖尔 - 高斯(LG)光束有很大不同。我们揭示,由于短电子轨迹导致的单原子固有相位可以通过BG光束的几何相位得到很好的补偿,从而可以在离轴且远离激光焦点的位置实现有利的相位匹配条件。因此,我们给出了一个通用规则:当气体介质位于BG光束激光焦点之前或之后1.5z至2.0z处时(这里z是约化长度),可以高效地产生具有单个环形分布的涡旋高次谐波。我们还展示了当BG光束携带更高OAM时该规则的有效性。这项工作有望对合成阿秒涡旋脉冲有用。

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