Li Yupeng, Wu Yi, Xu Chenchao, Liu Ningning, Ma Jiang, Lv Baijiang, Yao Gang, Liu Yan, Bai Hua, Yang Xiaohui, Qiao Lei, Li Miaocong, Li Linjun, Xing Hui, Huang Yaobo, Ma Junzhang, Shi Ming, Cao Chao, Liu Yang, Liu Canhua, Jia Jinfeng, Xu Zhu-An
Zhejiang Province Key Laboratory of Quantum Technology and Device, Department of Physics, Zhejiang University, Hangzhou 310027, China.
Key Laboratory of Artificial Structures and Quantum Control (Ministry of Education), Department of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai 200240, China.
Sci Bull (Beijing). 2021 Feb 15;66(3):243-249. doi: 10.1016/j.scib.2020.09.007. Epub 2020 Sep 8.
Topological materials and topological phases have recently become a hot topic in condensed matter physics. In this work, we report an In-intercalated transition-metal dichalcogenide InTaSe (named 112 system), a topological nodal-line semimetal in the presence of both charge density wave (CDW) and superconductivity. In the x = 0.58 sample, the 2×3 commensurate CDW (CCDW) and the 2×2 CCDW are observed below 116 and 77 K, respectively. Consistent with theoretical calculations, the spin-orbital coupling gives rise to two twofold-degenerate nodal rings (Weyl rings) connected by drumhead surface states, confirmed by angle-resolved photoemission spectroscopy. Our results suggest that the 2×2 CCDW ordering gaps out one Weyl ring in accordance with the CDW band folding, while the other Weyl ring remains gapless with intact surface states. In addition, superconductivity emerges at 0.91 K, with the upper critical field deviating from the s-wave behavior at low temperature, implying possibly unconventional superconductivity. Therefore, we think this type of the 112 system may possess abundant physical states and offer a platform to investigate the interplay between CDW, nontrivial band topology and superconductivity.
拓扑材料和拓扑相最近已成为凝聚态物理中的一个热门话题。在这项工作中,我们报道了一种铟插层的过渡金属二硫属化物InTaSe(命名为112体系),它是一种在存在电荷密度波(CDW)和超导性的情况下的拓扑节线半金属。在x = 0.58的样品中,分别在116 K和77 K以下观察到2×3相称CDW(CCDW)和2×2 CCDW。与理论计算一致,自旋轨道耦合产生了由鼓面表面态连接的两个双重简并节环(外尔环),这通过角分辨光电子能谱得到证实。我们的结果表明,2×2 CCDW有序化根据CDW能带折叠使一个外尔环带隙,而另一个外尔环在表面态完整的情况下仍然无带隙。此外,超导性在0.91 K出现,其高临界场在低温下偏离s波行为,这意味着可能存在非常规超导性。因此,我们认为这种类型的112体系可能具有丰富的物理态,并为研究CDW、非平凡能带拓扑和超导性之间的相互作用提供了一个平台。