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扫描透射电子显微镜中相位对比图像重建的优化探测器配置。

Optimized detector configurations for the reconstruction of phase-contrast images in scanning transmission electron microscopy.

机构信息

University of Münster (Westfälische Wilhelms-Universität Münster), Wilhelm Klemm Str. 10, 48149 Münster, Germany.

出版信息

Ultramicroscopy. 2023 Apr;246:113670. doi: 10.1016/j.ultramic.2022.113670. Epub 2023 Jan 12.

DOI:10.1016/j.ultramic.2022.113670
PMID:36657215
Abstract

Using the differential phase contrast mechanism and anti-symmetric detector geometries it is possible to image distributions of electric and magnetic fields in a scanning transmission electron microscope. Different detector geometries can be used for imaging and, due to their efficiency, mainly ring quadrant detectors and pixelated detectors have been used in recent high resolution differential phase contrast experiments. In 4D-Scanning Transmission Electron Microscopy one uses a pixelated (2D) detector to obtain the complete scattering distribution for every (2D) image point. The accuracy of pixelated detectors increases with an increasing number of pixels, which in turn also leads to a larger amount of data that needs to be evaluated. To reduce the required numerical effort, we are looking for alternative detector geometries by further segmenting ring quadrant detectors. To compare the different geometries, their signal-to-noise ratios are calculated for an ideal STEM and several weak phase objects. Images can be obtained by combining the data of different detector pixels using a scheme similar to a reconstruction from a focal series. The procedure can be interpreted as the simplest example of ptychography including only the first-order diffraction disks. Our results show that a 50-segment annular bright-field detector can reach a signal-to-noise ratio close to that of a 128 × 128 pixelated detector, while having a significantly lower number of segments that need to be evaluated.

摘要

利用差分相衬机制和反对称探测器几何形状,可以在扫描透射电子显微镜中成像电场和磁场的分布。可以使用不同的探测器几何形状进行成像,由于其效率,最近的高分辨率差分相衬实验主要使用环形象限探测器和像素化探测器。在 4D 扫描透射电子显微镜中,使用像素化(2D)探测器来获得每个(2D)图像点的完整散射分布。像素化探测器的精度随着像素数量的增加而增加,这反过来也导致需要评估的数据量增加。为了减少所需的数值工作量,我们正在通过进一步分割环形象限探测器来寻找替代的探测器几何形状。为了比较不同的几何形状,我们计算了理想 STEM 和几个弱相位物体的信噪比。可以通过使用类似于焦系列重建的方案来组合不同探测器像素的数据来获得图像。该过程可以解释为包括一阶衍射盘的最简单的相衬术示例。我们的结果表明,50 段环形明场探测器可以达到接近 128×128 像素化探测器的信噪比,而需要评估的段数明显减少。

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