Department of Electrical and Computer Engineering, University of Washington, Seattle, WA 98195, United States of America.
Nanotechnology. 2023 Feb 10;34(17). doi: 10.1088/1361-6528/acb5fb.
Metal halide perovskites are emerging materials for integrated photonics. Here we report a quasi-CW pumped ultra-low ASE/lasing threshold formamidinium lead bromide (FAPbBr) laser. The laser achieved stable lasing at 555 nm with a full width at half maximum (FWHM) of 0.6 nm, showing a low lasing threshold of 22.6J cmunder 3.5 nanosecond quasi-CW excitation at room temperature. The material also showed an ultra-low ASE threshold of 46J cmunder the same pumping condition. Through polymer doping, we showed that the material's performance can be improved by increasing bimolecular recombination rate with reduced grain size.
金属卤化物钙钛矿是集成光子学的新兴材料。在这里,我们报道了一种准连续波泵浦的超低 ASE/激光阈值甲脒碘化铅(FAPbBr)激光器。该激光器在室温下,在 3.5 纳秒准连续波激发下,以 0.6nm 的全宽半最大值(FWHM)实现了 555nm 的稳定激光,表现出 22.6J/cm 的低激光阈值。在相同的泵浦条件下,该材料还表现出超低的 ASE 阈值为 46J/cm。通过聚合物掺杂,我们表明通过增加双分子复合速率并减小晶粒尺寸,可以提高材料的性能。