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碳纳米管电子黑体及其辐射光谱。

Carbon nanotube electron blackbody and its radiation spectra.

机构信息

State Key Laboratory of Low Dimensional Quantum Physics, Department of Physics, Tsinghua University, Beijing 100084, China.

Tsinghua-Foxconn Nanotechnology Research Center, Tsinghua University, Beijing 100084, China.

出版信息

Proc Natl Acad Sci U S A. 2023 Feb 7;120(6):e2209670120. doi: 10.1073/pnas.2209670120. Epub 2023 Jan 31.

DOI:10.1073/pnas.2209670120
PMID:36719922
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC9963611/
Abstract

An optical blackbody is an ideal absorber for all incident optical radiation, and the theoretical study of its radiation spectra paved the way for quantum mechanics (Planck's law). Herein, we propose the concept of an electron blackbody, which is a perfect electron absorber as well as an electron emitter with standard energy spectra at different temperatures. Vertically aligned carbon nanotube arrays are electron blackbodies with an electron absorption coefficient of 0.95 for incident energy ranging from 1 keV to 20 keV and standard electron emission spectra that fit well with the free electron gas model. Such a concept might also be generalized to blackbodies for extreme ultraviolet, X-ray, and -ray photons as well as neutrons, protons, and other elementary particles.

摘要

光学黑体是所有入射光辐射的理想吸收体,其辐射光谱的理论研究为量子力学(普朗克定律)铺平了道路。在此,我们提出了电子黑体的概念,它既是完美的电子吸收体,也是在不同温度下具有标准能谱的电子发射体。垂直排列的碳纳米管阵列是电子黑体,对于入射能量在 1keV 到 20keV 之间的电子,其电子吸收率为 0.95,并且具有与自由电子气体模型吻合较好的标准电子发射谱。这一概念也可能推广到极紫外光、X 射线和伽马射线光子以及中子、质子和其他基本粒子的黑体。

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Carbon nanotube electron blackbody and its radiation spectra.碳纳米管电子黑体及其辐射光谱。
Proc Natl Acad Sci U S A. 2023 Feb 7;120(6):e2209670120. doi: 10.1073/pnas.2209670120. Epub 2023 Jan 31.
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本文引用的文献

1
Large-Area and Broadband Thermoelectric Infrared Detection in a Carbon Nanotube Black-Body Absorber.碳纳米管黑体吸收器中的大面积宽带热电热红外探测
ACS Nano. 2019 Nov 26;13(11):13285-13292. doi: 10.1021/acsnano.9b06332. Epub 2019 Nov 15.
2
Evidence for a Quasi-One-Dimensional Charge Density Wave in CuTe by Angle-Resolved Photoemission Spectroscopy.角分辨光电子能谱研究 CuTe 中的准一维电荷密度波。
Phys Rev Lett. 2018 Nov 16;121(20):206402. doi: 10.1103/PhysRevLett.121.206402.
3
Extremely Black Vertically Aligned Carbon Nanotube Arrays for Solar Steam Generation.
用于太阳能蒸汽发生的超黑垂直排列碳纳米管阵列。
ACS Appl Mater Interfaces. 2017 Aug 30;9(34):28596-28603. doi: 10.1021/acsami.7b08619. Epub 2017 Aug 16.
4
Direct Synthesis of Graphdiyne Nanowalls on Arbitrary Substrates and Its Application for Photoelectrochemical Water Splitting Cell.在任意衬底上直接合成石墨炔纳米墙及其在光电化学水分解电池中的应用。
Adv Mater. 2017 Mar;29(9). doi: 10.1002/adma.201605308. Epub 2016 Dec 23.
5
Synthesis of Graphdiyne Nanowalls Using Acetylenic Coupling Reaction.使用炔偶联反应合成石墨炔纳米墙。
J Am Chem Soc. 2015 Jun 24;137(24):7596-9. doi: 10.1021/jacs.5b04057. Epub 2015 Jun 10.
6
Carbon nanotube-based tandem absorber with tunable spectral selectivity: transition from near-perfect blackbody absorber to solar selective absorber.基于碳纳米管的串联吸收体,具有可调谐的光谱选择性:从近完美黑体吸收体到太阳能选择性吸收体的转变。
Adv Mater. 2014 Apr 23;26(16):2552-7. doi: 10.1002/adma.201305070. Epub 2014 Jan 28.
7
Very black infrared detector from vertically aligned carbon nanotubes and electric-field poling of lithium tantalate.基于垂直定向碳纳米管和钽酸锂电场极化的深紫外探测器。
Nano Lett. 2010 Sep 8;10(9):3261-6. doi: 10.1021/nl100582j.
8
A black body absorber from vertically aligned single-walled carbon nanotubes.一种由垂直排列的单壁碳纳米管制成的黑体吸收器。
Proc Natl Acad Sci U S A. 2009 Apr 14;106(15):6044-7. doi: 10.1073/pnas.0900155106. Epub 2009 Apr 1.
9
Measuring the work function of carbon nanotubes with thermionic method.用热电子发射法测量碳纳米管的功函数。
Nano Lett. 2008 Feb;8(2):647-51. doi: 10.1021/nl0730817. Epub 2008 Jan 29.
10
Experimental observation of an extremely dark material made by a low-density nanotube array.由低密度纳米管阵列制成的极暗材料的实验观察
Nano Lett. 2008 Feb;8(2):446-51. doi: 10.1021/nl072369t. Epub 2008 Jan 9.