Geng Haopeng, Zhang Jian, Xie Rong, Dai Songbo, Pan Baotian
Key Laboratory of Western China's Environmental Systems (Ministry of Education), College of Earth and Environmental Sciences, Lanzhou University, Lanzhou 730000, China; Shiyang River Basin Scientific Observing Station of Gansu Province, Lanzhou 730000, China.
Key Laboratory of Western China's Environmental Systems (Ministry of Education), College of Earth and Environmental Sciences, Lanzhou University, Lanzhou 730000, China.
Sci Total Environ. 2023 Apr 20;870:161946. doi: 10.1016/j.scitotenv.2023.161946. Epub 2023 Feb 2.
Quantifying the relationship between the chemical weathering and denudation rates of active orogenic belts over a range of climates is the key to addressing the controversy over the uplift-weathering hypothesis. However, studies have focused on warm and humid environments and have not examined cold and arid environments. Here, we present a new dataset of the chemical depletion fraction (CDF: ratio of the chemical weathering rate to the total denudation rate) across the arid to semiarid Qilian Mountains on the northeastern Tibetan Plateau, where the uplift-weathering hypothesis has been proposed. We selected 60 points from 12 catchments in the middle Qilian Mountains. At each point, we collected three samples (soil, saprolite, and bedrock samples) and calculated the CDF values based on their Zr concentrations. We found no clear correlation between the CDF and climatic factors (temperature, precipitation, and normalized difference vegetation index (NDVI)), topographic factors (slope and local relief), and denudation rate. The calculated chemical weathering rates, nevertheless, are positively correlated with precipitation, NDVI, and denudation rate, and negatively correlated with temperature. This result indicates that the Qilian Mountains are under supply-limited conditions, even at high denudation rates (>800 t km y). We speculate that low temperatures (<0 °C) could intensify near-surface chemical weathering by promoting the physical breakdown of the bedrock and increasing soil water availability. This mechanism causes a compensation effect maintaining the supply-limited conditions in landscapes with high denudation rates. Combing a worldwide dataset regarding the correlations between CDF and climatic factors and denudation rates, we argue that intensified denudation since the late Cenozoic contributed to global cooling.
量化不同气候条件下活动造山带化学风化与剥蚀速率之间的关系,是解决隆升 - 风化假说争议的关键。然而,以往研究主要集中在温暖湿润环境,尚未涉及寒冷干旱环境。在此,我们展示了青藏高原东北部干旱至半干旱祁连山脉的化学损耗分数(CDF:化学风化速率与总剥蚀速率之比)的新数据集,该地区已提出隆升 - 风化假说。我们从祁连山中段的12个流域选取了60个点。在每个点,我们采集了三个样本(土壤、风化层和基岩样本),并根据它们的锆浓度计算了CDF值。我们发现CDF与气候因素(温度、降水和归一化植被指数(NDVI))、地形因素(坡度和局部地形起伏)以及剥蚀速率之间没有明显的相关性。然而,计算得出的化学风化速率与降水、NDVI和剥蚀速率呈正相关,与温度呈负相关。这一结果表明,即使在高剥蚀速率(>800 t km² y⁻¹)下,祁连山脉仍处于供应受限的条件。我们推测,低温(<0°C)可能通过促进基岩的物理破碎和增加土壤水分有效性来强化近地表化学风化。这种机制产生了一种补偿效应,在高剥蚀速率的地貌中维持供应受限的条件。结合全球范围内关于CDF与气候因素和剥蚀速率之间相关性的数据集,我们认为新生代晚期以来剥蚀作用的增强促成了全球变冷。