Univ. Lille, Institut Mines-Télécom, Univ. Artois, Junia, ULR 4515 - LGCgE, Laboratoire de Génie Civil et géo-Environnement, F-59000, Lille, France.
Univ. Lille, Institut Mines-Télécom, Univ. Artois, Junia, ULR 4515 - LGCgE, Laboratoire de Génie Civil et géo-Environnement, F-59000, Lille, France.
Environ Pollut. 2023 Apr 1;322:121212. doi: 10.1016/j.envpol.2023.121212. Epub 2023 Feb 3.
Plastic waste and its fragments (microplastics; <5 mm) have been observed in almost all types of environments. However, the mechanisms underlying the flow and transport processes of plastics are unknown. This is particularly valid for river sediments, where complex interactions occur between particles and influence their vertical and horizontal distribution patterns. In this study, we investigated the vertical redistribution of 14 pristine microplastics (MPs) with different densities, sizes, and shapes within disturbed sediment without lateral transport (i.e., low-velocity flow). MPs were spiked into sediments (height: 8 cm) in a column with a height of 1 m (diameter: 6 cm) filled to the top with water. The sediment was perturbed by turning the column upside-down to simulate remobilization and the subsequent deposition of sediment. After the complete sedimentation of the particles, the water column was filtered and the sediment was cut into vertical sections. MPs were then extracted from the sediment using sieves and a density separation method, and were counted under a stereomicroscope. Low-density polymers were mainly recovered in the water column and at the surface of the sediment, whereas high-density polymers were found within all sediment sections. The vertical distribution of high-density polymers changes primarily with the sediment grain size. The distribution of each polymer type changes depending on the size and/or shape of the particles with complex interactions. The observed distributions were compared with the expected distributions based only on the vertical velocity formulas. Overall, the formulas used did not explain the sedimentation of a portion of low-density polymers and predicted a lower distribution in the sediment than those observed in the experiment. In conclusion, this study highlights the importance of considering MPs as multi-dimensional particles and provides clues to understand their fate in low-velocity flow systems, considering that they undergo scavenging in sediments.
塑料废物及其碎片(微塑料;<5 毫米)几乎存在于所有类型的环境中。然而,塑料的流动和输运过程的机制尚不清楚。这在河流沉积物中尤其如此,其中颗粒之间存在复杂的相互作用,影响它们的垂直和水平分布模式。在这项研究中,我们研究了在没有侧向输运(即低流速)的情况下,不同密度、大小和形状的 14 种原始微塑料(MPs)在受扰沉积物中的垂直再分布。将 MPs 加入到 1 米高(直径:6 厘米)的柱子中,柱子的高度为 8 厘米,装满水。通过将柱子倒置来模拟再悬浮和随后的沉积物沉积,从而扰动沉积物。在颗粒完全沉降后,过滤水柱,将沉积物切成垂直段。然后使用筛子和密度分离法从沉积物中提取 MPs,并在立体显微镜下计数。低密度聚合物主要回收在水柱和沉积物表面,而高密度聚合物则存在于所有沉积物段中。高密度聚合物的垂直分布主要随沉积物粒径而变化。每种聚合物类型的分布取决于颗粒的大小和/或形状,存在复杂的相互作用。观察到的分布与仅基于垂直速度公式的预期分布进行了比较。总体而言,使用的公式不能解释部分低密度聚合物的沉降,并且预测的沉积物中的分布低于实验中观察到的分布。总之,本研究强调了将 MPs 视为多维颗粒的重要性,并提供了了解它们在低流速流动系统中的命运的线索,因为它们在沉积物中会被清除。