Zhang Zhen, Yang Zenan, Zhao Zhixi, Liu Yiyang, Wang Chenchong, Xu Wei
State Key Laboratory of Rolling and Automation, School of Materials Science and Engineering, Northeastern University, Shenyang, Liaoning 110819, China.
Science and Technology on Advanced High Temperature Structural Materials Laboratory, Beijing Institute of Aeronautical Materials, Beijing 100095, China.
ACS Appl Mater Interfaces. 2023 Feb 22;15(7):10261-10272. doi: 10.1021/acsami.2c21439. Epub 2023 Feb 12.
The lengthy process through which laser-textured surfaces transform from hydrophilic to hydrophobic severely restricts their practical applications. Accurately predicting the wettability evolution curve is crucial; however, developing a reliable prediction model remains challenging. Herein, a data-driven multimodal deep-learning framework was developed, in which multimodal data of micro/nanostructure morphology images, composition distribution images, and time information are effectively coupled and fed into a convolutional neural network (CNN). Rich data input and in-depth data mining make the framework more robust, achieving accurate prediction of the wettability evolution curves of various typical micro/nanostructures. Additionally, accurate prediction of input images with varying magnifications and untrained laser-textured surfaces demonstrates the generalizability of the multimodal CNN framework. The visualization results of the convolution layer confirmed the rationality of the information learned by the model. Additionally, the proposed multimodal CNN framework was successfully utilized to investigate the optimization process. Further, a laser-textured surface with a shorter evolution period and a larger final contact angle was realized. The proposed multimodal CNN framework offers an efficient and cost-effective method for predicting the wettability evolution curves and exploring the optimization processes, enhancing the application potential of laser micro/nanofabrication of superhydrophobic surfaces.
激光纹理表面从亲水性转变为疏水性的漫长过程严重限制了它们的实际应用。准确预测润湿性演变曲线至关重要;然而,开发一个可靠的预测模型仍然具有挑战性。在此,开发了一种数据驱动的多模态深度学习框架,其中微/纳米结构形态图像、成分分布图像和时间信息的多模态数据被有效地耦合,并输入到卷积神经网络(CNN)中。丰富的数据输入和深入的数据挖掘使该框架更加稳健,能够准确预测各种典型微/纳米结构的润湿性演变曲线。此外,对具有不同放大倍数的输入图像和未训练的激光纹理表面进行准确预测,证明了多模态CNN框架的通用性。卷积层的可视化结果证实了模型所学习信息的合理性。此外,所提出的多模态CNN框架成功地用于研究优化过程。进一步实现了具有更短演变周期和更大最终接触角的激光纹理表面。所提出的多模态CNN框架为预测润湿性演变曲线和探索优化过程提供了一种高效且经济高效的方法,增强了超疏水表面激光微/纳米制造的应用潜力。