在双金属层状双氢氧化物中产生氧空位用于水氧化的通用策略。
A general strategy to generate oxygen vacancies in bimetallic layered double hydroxides for water oxidation.
作者信息
Wu Konglin, Shi Luoxiang, Wang Zhendong, Zhu Ye, Tong Xinyue, He Wenxiang, Wang Junwei, Zheng Lirong, Kang Yanshang, Shan Weilong, Wang Zhiguo, Huang Aijian, Jiang Binbin
机构信息
Engineering Research Center of Biofilm Water Purification and Utilization Technology of Ministry of Education, Anhui University of Technology, Maanshan, 243032, China.
Anhui Laboratory of Molecule-Based Materials, College of Chemistry and Materials Science, Anhui Normal University, Wuhu, 241002, China.
出版信息
Chem Commun (Camb). 2023 Mar 9;59(21):3138-3141. doi: 10.1039/d3cc00096f.
A general electrocatalyst design for water splitting through generating oxygen vacancies in bimetallic layered double hydroxides by using carbon nitride is proposed. The excellent OER activity of the achieved bimetallic layered double hydroxides is attributed to oxygen vacancies, which reduce the energy barrier of the rate-determining step.
提出了一种通过使用氮化碳在双金属层状双氢氧化物中产生氧空位来进行水分解的通用电催化剂设计。所制备的双金属层状双氢氧化物优异的析氧反应活性归因于氧空位，其降低了速率决定步骤的能垒。
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