Faculty of Chemistry, Bu-Ali Sina University, Hamedan, Iran.
School of Chemistry, University of Melbourne, Victoria 3010, Australia.
Dalton Trans. 2023 May 30;52(21):7031-7047. doi: 10.1039/d3dt00256j.
Tris(2-aminoethyl)amine (tren) coordinates to a Zn(II) ion to form the [Zn(tren)] cation that accepts a monodentate favipiravir (FAV) anion. The results of this work show that the FAV anion is capable of binding to the [Zn(tren)] cation through either a nitrogen or an oxygen atom (/-coordination). The energy decomposition analysis shows that, interestingly, both the strength and nature of the bonds between the [Zn(tren)] cation and the /-coordinated FAV anion are almost the same. X-ray crystal structure determinations confirmed the existence of two types of cations in the solid state, [Zn(tren)(-FAV)] and [Zn(tren)(-FAV)]. The NMR data, in a DMSO solution, were consistent with either the -coordinated or the -coordinated complex, but not a mixture of the two linkage isomers. The theoretical data indicated that the [Zn(tren)(-FAV)] and [Zn(tren)(-FAV)] cations have very similar stability in the gas phase, and in HO, CHOH, and DMSO solutions, and can also easily convert from one linkage isomer to the other. The experimental and theoretical data showed that, upon protonation of the above cations under acidic conditions (pH ≈ 3 to 5.5), the drug FAV will be easily released and replaced by a Cl anion, or an HO molecule, which will coordinate to the zinc atom showing the potential of [Zn(tren)] as a safe drug vehicle. Molecular docking studies using two well-known molecular docking packages show the relatively strong binding interactions of the [Zn(tren)(-FAV)] and [Zn(tren)(-FAV)] cations with DNA and viral protein macromolecules.
三(2-氨基乙基)胺(tren)与 Zn(II) 离子配位形成 [Zn(tren)] 阳离子,该阳离子接受一个单价的法匹拉韦(FAV)阴离子。这项工作的结果表明,FAV 阴离子能够通过氮原子或氧原子(/-配位)与 [Zn(tren)] 阳离子结合。能量分解分析表明,有趣的是,[Zn(tren)] 阳离子与/-配位的 FAV 阴离子之间的键的强度和性质几乎相同。X 射线晶体结构测定证实了在固态中存在两种类型的阳离子,[Zn(tren)(-FAV)] 和 [Zn(tren)(-FAV)]。在 DMSO 溶液中的 NMR 数据与/-配位或/-配位的配合物一致,但不是两种连接异构体的混合物。理论数据表明,[Zn(tren)(-FAV)] 和 [Zn(tren)(-FAV)] 阳离子在气相中、在 HO、CHOH 和 DMSO 溶液中具有非常相似的稳定性,并且可以很容易地从一种连接异构体转化为另一种。实验和理论数据表明,在酸性条件下(pH ≈ 3 至 5.5)对上述阳离子进行质子化时,药物 FAV 将很容易释放并被 Cl 阴离子或 HO 分子取代,这些分子将与锌原子配位,显示出 [Zn(tren)] 作为安全药物载体的潜力。使用两个著名的分子对接包进行的分子对接研究表明,[Zn(tren)(-FAV)] 和 [Zn(tren)(-FAV)] 阳离子与 DNA 和病毒蛋白大分子具有相对较强的结合相互作用。