Liu Xianchao, Zhang Zhiheng, Han Chao, Wu Jiang, Zhang Xingchao, Zhou Hongxi, Xie Qian, Wang Jun
School of Optoelectronic Science and Engineering, University of Electronic Science and Technology of China, Chengdu, 610054, China.
Institute of Fundamental and Frontier Sciences, University of Electronic Science and Technology of China, Chengdu, 610054, China.
Discov Nano. 2023 Mar 8;18(1):35. doi: 10.1186/s11671-023-03817-5.
Broadband high absorption of long-wavelength infrared light for rough submicron active material films is quite challenging to achieve. Unlike conventional infrared detection units, with over three-layer complex structures, a three-layer metamaterial with mercury cadmium telluride (MCT) film sandwiched between an Au cuboid array and Au mirror is studied through theory and simulations. The results show that propagated/localized surface plasmon resonance simultaneously contribute to broadband absorption under the TM wave of the absorber, while the Fabry-Perot (FP) cavity resonance causes absorption of the TE wave. As surface plasmon resonance concentrates most of the TM wave on the MCT film, 74% of the incident light energy is absorbed by the submicron thickness MCT film within the 8-12 μm waveband, which is approximately 10 times than that of the rough same thickness MCT film. In addition, by replacing the Au mirror with Au grating, the FP cavity along the y-axis direction was destroyed, and the absorber exhibited excellent polarization-sensitive and incident angle-insensitive properties. For the corresponding conceived metamaterial photodetector, as carrier transit time across the gap between Au cuboid is much less than that of other paths, the Au cuboids simultaneously act as microelectrodes to collect photocarriers generated in the gap. Thus the light absorption and photocarrier collection efficiency are hopefully improved simultaneously. Finally, the density of the Au cuboids is increased by adding the same arranged cuboids perpendicular to the original direction on the top surface or by replacing the cuboids with crisscross, which results in broadband polarization-insensitive high absorption by the absorber.
实现粗糙亚微米活性材料薄膜对长波长红外光的宽带高吸收颇具挑战性。与具有三层以上复杂结构的传统红外探测单元不同,本文通过理论和模拟研究了一种三层超材料,其结构为在金长方体阵列和金镜之间夹有碲镉汞(MCT)薄膜。结果表明,传播型/局域表面等离子体共振同时有助于吸收体TM波下的宽带吸收,而法布里-珀罗(FP)腔共振导致TE波的吸收。由于表面等离子体共振将大部分TM波集中在MCT薄膜上,在8-12μm波段内,亚微米厚度的MCT薄膜吸收了74%的入射光能,这大约是相同厚度粗糙MCT薄膜的10倍。此外,用金光栅代替金镜,破坏了沿y轴方向的FP腔,吸收体表现出优异的偏振敏感和入射角不敏感特性。对于相应的超材料光电探测器,由于载流子穿过金长方体之间间隙的渡越时间远小于其他路径,金长方体同时充当微电极来收集间隙中产生的光载流子。因此有望同时提高光吸收和光载流子收集效率。最后,通过在顶表面垂直于原始方向添加相同排列的长方体或用交叉长方体代替长方体来增加金长方体的密度,这使得吸收体实现宽带偏振不敏感高吸收。