Laboratoire de Physique des Solides, CNRS, Université Paris-Saclay, 91405 Orsay, France.
Constructive Solutions for Science and Technology, 33649 Bielefeld, Germany.
Rev Sci Instrum. 2023 Mar 1;94(3):037102. doi: 10.1063/5.0137762.
We reply to the Comment by Donath et al. on our setup, which allows a total 3D control of the polarization direction of the electron beam in an inverse photoemission spectroscopy (IPES) experiment, a significant advance with respect to previous setups with partial polarization control. Donath et al. claim an incorrect operation of our setup after comparing their results, treated to enhance the spin asymmetry, with our spectra without the same treatment. They also equal spectra backgrounds instead of equaling peak intensities above the background. Thus, we compare our Cu(001) and Au(111) results with the literature. We reproduce previous results, including spin-up/spin-down spectral differences observed for Au and not observed for Cu. Also, spin-up/spin-down spectral differences appear at the expected reciprocal space regions. In the Comment, it is also stated that our tuning of the spin polarization misses the target because the spectra background changes when tuning the spin. We argue that the background change is irrelevant to IPES since the information is contained in peaks produced by primary electrons, those having conserved their energy in the inverse photoemission process. Second, our experiments agree with previous results from Donath et al. [Wissing et al., New J. Phys. 15, 105001 (2013)] and with a zero-order quantum-mechanical model of spins in vacuum. Deviations are explained by more realistic descriptions including the spin transmission through an interface. Consequently, the operation of our original setup is fully demonstrated. Our development corresponds to "the promising and rewarding angle-resolved IPES setup with the three-dimensional spin resolution," as indicated in the Comment, after our work.
我们回复了 Donath 等人对我们的实验设置的评论,该设置允许在逆光电发射谱 (IPES) 实验中完全控制电子束的极化方向,与具有部分极化控制的先前设置相比是一个重大进展。Donath 等人声称在比较他们的结果(经过处理以增强自旋不对称性)与我们未经相同处理的光谱后,我们的设置操作不正确。他们还将光谱背景相等而不是将背景上方的峰值强度相等。因此,我们将我们的 Cu(001) 和 Au(111) 结果与文献进行比较。我们再现了以前的结果,包括在 Au 中观察到的而在 Cu 中未观察到的自旋向上/向下谱差异。此外,自旋向上/向下谱差异出现在预期的倒空间区域。在评论中,还指出我们的自旋极化调节未达到目标,因为在调节自旋时光谱背景会发生变化。我们认为背景变化与 IPES 无关,因为信息包含在由初级电子产生的峰中,这些电子在逆光电发射过程中保持了能量。其次,我们的实验与 Donath 等人的先前结果[Wissing 等人,New J. Phys. 15, 105001 (2013)]以及真空中自旋的零阶量子力学模型一致。偏差可以通过更现实的描述来解释,包括通过界面的自旋传输。因此,我们原始设置的操作得到了充分证明。我们的发展对应于评论中指出的“具有三维自旋分辨率的有前途和有益的角分辨 IPES 设置”,这是在我们的工作之后。