Luo Guoqiang, Cheng Pu, Yu Yin, Geng Xiangwei, Zhao Yue, Xia Yulong, Zhang Ruizhi, Shen Qiang
Chaozhou Branch of Chemistry and Chemical Engineering Guangdong Laboratory, Chaozhou 521000, China.
State Key Lab of Advanced Technology for Materials Synthesis and Processing, Wuhan University of Technology, Wuhan 430070, China.
Polymers (Basel). 2023 Mar 28;15(7):1680. doi: 10.3390/polym15071680.
Particulate polymer composites (PPCs) are widely applied under different elastic wave loading conditions in the automobile, aviation, and armor protection industries. This study investigates the elastic wave propagation behavior of a typical PPC, specifically a Cu/poly (methyl methacrylate) () composite, with a wide range of particle contents (30-65 vol. %) and particle sizes (1-100 μm). The results demonstrate an inflection phenomenon in both the elastic wave velocity and attenuation coefficient with increasing volume content. In addition, the inflection point moves to the direction of low content with the increase in particle size. Notably, the elastic wave velocity, attenuation, and wavefront width significantly increased with the particle size. The inflection phenomenon of elastic wave propagation behavior in PPCs is demonstrated to have resulted from particle interaction using the classical scattering theory and finite element analysis. The particle interaction initially intensified and then reduced with increasing particle content. This study elucidates the underlying mechanism governing the elastic wave propagation behavior of high particle content PPCs and provides guidelines for the design and application of wave-absorbing composites.
颗粒聚合物复合材料(PPCs)在汽车、航空和装甲防护行业的不同弹性波加载条件下得到了广泛应用。本研究调查了一种典型的PPC,即铜/聚甲基丙烯酸甲酯()复合材料在广泛的颗粒含量(30 - 65体积%)和颗粒尺寸(1 - 100微米)范围内的弹性波传播行为。结果表明,随着体积含量的增加,弹性波速度和衰减系数均出现拐点现象。此外,随着颗粒尺寸的增加,拐点向低含量方向移动。值得注意的是,弹性波速度、衰减和波前宽度随颗粒尺寸显著增加。利用经典散射理论和有限元分析表明,PPCs中弹性波传播行为的拐点现象是由颗粒相互作用引起的。颗粒相互作用最初随着颗粒含量的增加而增强,然后减弱。本研究阐明了高颗粒含量PPCs弹性波传播行为的潜在机制,并为吸波复合材料的设计和应用提供了指导。