MIIT Key Laboratory of Advanced Display Materials and Devices, Institute of Optoelectronics & Nanomaterials, School of Materials Science and Engineering, Nanjing University of Science and Technology, Nanjing 210094, China.
Chem Commun (Camb). 2023 May 2;59(36):5365-5374. doi: 10.1039/d2cc06534g.
Metal halide perovskite nanocrystals (NCs) have been widely studied for application in photonics and optoelectronics due to their excellent photoelectric properties. Perovskite NCs with narrow luminescence linewidth and high photoluminescence quantum yield are excellent assembly modules for building large-scale NC superlattices. The coupling of optics and electricity in such excellent aggregates gives them exceptional collective photoelectric performance, such as superfluorescence, red-shifted emission, coupling-enhanced electron transport, Perovskite NC superlattices are expected to become another hot research topic in optoelectronics. Here, we focus on the collective behavior of superlattices and review the recent progress of the self-assembly, collective photoelectric properties, and applications of perovskite NC superlattices. Finally, a few challenges and prospects are indicated.
金属卤化物钙钛矿纳米晶体(NCs)由于其优异的光电性能,已被广泛研究应用于光子学和光电领域。具有窄发光线宽和高光致发光量子产率的钙钛矿 NCs 是构建大规模 NC 超晶格的优秀组装模块。这种优异的聚集体中光学和电学的耦合赋予了它们非凡的集体光电性能,如超荧光、发射红移、耦合增强的电子输运等。钙钛矿 NC 超晶格有望成为光电领域的另一个热门研究课题。在这里,我们重点关注超晶格的集体行为,并综述了钙钛矿 NC 超晶格的自组装、集体光电特性和应用的最新进展。最后,指出了一些挑战和展望。