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二维狄拉克晶体中与声子强烈相关的电子的动态介电函数和声子自能。

Dynamic dielectric function and phonon self-energy from electrons strongly correlated with acoustic phonons in 2D Dirac crystals.

机构信息

Department of Physics and Astronomy, The University of Western Ontario, London, ON, Canada.

出版信息

J Phys Condens Matter. 2023 May 11;35(32). doi: 10.1088/1361-648X/acceee.

Abstract

The unique structure of two-dimensional (2D) Dirac crystals, with electronic bands linear in the proximity of the Brillouin-zone boundary and the Fermi energy, creates anomalous situations where small Fermi-energy perturbations critically affect the electron-related lattice properties of the system. The Fermi-surface nesting (FSN) conditions determining such effects via electron-phonon interaction require accurate estimates of the crystal's response function(χ)as a function of the phonon wavevectorfor any values of temperature, as well as realistic hypotheses on the nature of the phonons involved. Numerous analytical estimates ofχ(q)for 2D Dirac crystals beyond the Thomas-Fermi approximation have been so far carried out only in terms of dielectric response functionχ(q,ω), for photon and optical-phonon perturbations, due to relative ease of incorporating a-independent oscillation frequency(ω)in calculation. Models accounting for Dirac-electron interaction with acoustic phonons, for whichis linear toand is therefore dispersive, are essential to understand many critical crystal properties, including electrical and thermal transport. The lack of such models has often led to the assumption that the dielectric response functionχ(q)in these systems can be understood from free-electron behavior. Here, we show that, different from free-electron systems,χ(q)calculated for acoustic phonons in 2D Dirac crystals using the Lindhard model, exhibits a cuspidal point at the FSN condition. Strong variability of∂χ∂qpersists also at finite temperatures, whileχ(q)tend to infinity in the dynamic case where the speed of sound is small, albeit non negligible, over the Dirac-electron Fermi velocity. The implications of our findings for electron-acoustic phonon interaction and transport properties such as the phonon line width derived from the phonon self-energy will also be discussed.

摘要

二维 (2D) 狄拉克晶体的独特结构,其电子能带在布里渊区边界和费米能附近呈线性,这创造了异常情况,即小的费米能微扰对系统的电子相关晶格性质产生至关重要的影响。通过电子-声子相互作用确定这种效应的费米面嵌套(FSN)条件要求准确估计晶体的响应函数 χ(q)作为声子波矢的函数,对于任何温度值,以及对所涉及的声子的性质的现实假设。迄今为止,对于托马斯-费米近似之外的二维狄拉克晶体,已经进行了大量 χ(q)的解析估计,仅在光频和光学声子微扰的介电响应函数 χ(q,ω)方面进行了计算,因为在计算中相对容易包含与 a 无关的振荡频率 (ω)。考虑到狄拉克电子与声学声子相互作用的模型,由于与成正比,因此是色散的,对于理解许多关键晶体性质,包括电输运和热输运,是必不可少的。缺乏这种模型通常导致假设这些系统中的介电响应函数 χ(q)可以从自由电子行为来理解。在这里,我们表明,与自由电子系统不同,使用林哈特模型计算的二维狄拉克晶体中的声学声子的 χ(q)在 FSN 条件下表现出尖点。在有限温度下, ∂χ∂q 的强变化也持续存在,而在声速在狄拉克电子费米速度下较小但非零的动态情况下, χ(q)趋于无穷大。我们的发现对电子-声学声子相互作用和输运性质的影响,例如从声子自能得出的声子线宽,也将进行讨论。

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