Jiang Xiangyi, Huang Boshi, Rumrill Shawn, Pople David, Zalloum Waleed A, Kang Dongwei, Zhao Fabao, Ji Xiangkai, Gao Zhen, Hu Lide, Wang Zhao, Xie Minghui, De Clercq Erik, Ruiz Francesc X, Arnold Eddy, Pannecouque Christophe, Liu Xinyong, Zhan Peng
Department of Medicinal Chemistry, Key Laboratory of Chemical Biology (Ministry of Education), School of Pharmaceutical Sciences, Cheeloo College of Medicine, Shandong University, 44 West Culture Road, Jinan, 250012, Shandong, PR China.
Center for Advanced Biotechnology and Medicine, Rutgers University, Piscataway, NJ, 08854, USA.
Commun Chem. 2023 Apr 29;6(1):83. doi: 10.1038/s42004-023-00888-4.
HIV-1 reverse transcriptase is one of the most attractive targets for the treatment of AIDS. However, the rapid emergence of drug-resistant strains and unsatisfactory drug-like properties seriously limit the clinical application of HIV-1 non-nucleoside reverse transcriptase inhibitors (NNRTIs). Here we show that a series of piperazine sulfonyl-bearing diarylpyrimidine-based NNRTIs were designed to improve the potency against wild-type and NNRTI-resistant strains by enhancing backbone-binding interactions. Among them, compound 18b1 demonstrates single-digit nanomolar potency against the wild-type and five mutant HIV-1 strains, which is significantly better than the approved drug etravirine. The co-crystal structure analysis and molecular dynamics simulation studies were conducted to explain the broad-spectrum inhibitory activity of 18b1 against reverse transcriptase variants. Besides, compound 18b1 demonstrates improved water solubility, cytochrome P450 liability, and other pharmacokinetic properties compared to the currently approved diarylpyrimidine (DAPY) NNRTIs. Therefore, we consider compound 18b1 a potential lead compound worthy of further study.
HIV-1逆转录酶是治疗艾滋病最具吸引力的靶点之一。然而,耐药菌株的迅速出现以及不尽人意的类药性质严重限制了HIV-1非核苷类逆转录酶抑制剂(NNRTIs)的临床应用。在此我们表明,设计了一系列含哌嗪磺酰基的二芳基嘧啶类NNRTIs,通过增强主链结合相互作用来提高对野生型和耐NNRTI菌株的效力。其中,化合物18b1对野生型和五种突变HIV-1菌株表现出个位数纳摩尔的效力,明显优于已获批药物依曲韦林。进行了共晶体结构分析和分子动力学模拟研究,以解释18b1对逆转录酶变体的广谱抑制活性。此外,与目前获批的二芳基嘧啶(DAPY)类NNRTIs相比,化合物18b1表现出改善的水溶性、细胞色素P450易感性及其他药代动力学性质。因此,我们认为化合物18b1是一个值得进一步研究的潜在先导化合物。