Centre for Nano Science and Engineering, Indian Institute of Science, Bangalore 560012, India.
Centre for Nano Science and Engineering, Indian Institute of Science, Bangalore 560012, India.
J Colloid Interface Sci. 2023 Sep 15;646:606-615. doi: 10.1016/j.jcis.2023.05.067. Epub 2023 May 16.
Interfacial instabilities cause undesirable droplet breakage during impact. Such breakage affects many applications, such as printing, spraying, etc. Particle coating over a droplet can significantly change the impact process and stabilize it against breakage. This work investigates the impact dynamics of particle-coated droplets, which mostly remains unexplored.
Particle-coated droplets of different mass loading were formed using volume addition. The prepared droplets were impacted on superhydrophobic surfaces, and their dynamics were recorded using a high-speed camera.
We report an intriguing phenomenon where an interfacial fingering instability helps suppress pinch-off in particle-coated droplets. This island of breakage suppression, where the droplet maintains its intactness upon impact, appears in a regime of Weber numbers where bare droplet breakage is inevitable. The onset of fingering instability in particle-coated droplets is observed at much lower impact energy, around two times less than the bare droplet. The instability is characterized and explained using the rim Bond number. The instability suppresses pinch-off because of the higher losses associated with the formation of stable fingers. Such instability can also be seen in dust/pollen-covered surfaces, making it useful in many applications related to cooling, self-cleaning, anti-icing etc.
界面不稳定性会导致在撞击过程中产生不良的液滴破碎。这种破碎会影响许多应用,如印刷、喷涂等。在液滴上覆盖颗粒可以显著改变撞击过程,并防止其破碎。这项工作研究了颗粒涂层液滴的撞击动力学,这方面的研究还很少。
使用体积添加的方法制备了不同质量负载的颗粒涂层液滴。制备好的液滴在超疏水表面上撞击,并使用高速摄像机记录它们的动力学。
我们报告了一个有趣的现象,即在颗粒涂层液滴中,界面指状不稳定性有助于抑制缩颈。在这种无破碎的断裂抑制岛中,液滴在撞击时保持完整,这出现在韦伯数的一个区域,在这个区域中,裸液滴必然会破碎。在颗粒涂层液滴中观察到指状不稳定性的出现所需的冲击能要低得多,大约是裸液滴的两倍。通过边缘邦德数来对不稳定性进行了特征描述和解释。不稳定性抑制了缩颈,因为与形成稳定的指状结构相关的能量损失更高。这种不稳定性也可以在尘土/花粉覆盖的表面上看到,因此在许多与冷却、自清洁、防冰等相关的应用中很有用。