Opt Lett. 2022 Dec 1;47(23):6241-6244. doi: 10.1364/OL.476994.
Based on the multipole expansion theory, we show that a transverse optical torque acting on a dipolar plasmonic spherical nanoparticle can be anomalously enhanced in two plane waves with linear polarization. Compared with a homogeneous Au nanoparticle, the transverse optical torque acting on an Au-Ag core-shell nanoparticle with an ultra-thin shell thickness can be dramatically enhanced by more than two orders of magnitude. Such enhanced transverse optical torque is dominated by the interaction between the incident optical field and the electric quadrupole excited in the dipolar core-shell nanoparticle. It is thus noted that the torque expression based on the dipole approximation usually used for dipolar particles is not available even in our dipolar case. These findings deepen the physical understanding of the optical torque (OT) and may have applications in optically driven rotation of plasmonic microparticles.
基于多极展开理论,我们表明,在具有线性偏振的两个平面波中,作用在偶极等离子体球形纳米粒子上的横向光扭矩可以异常增强。与均匀的 Au 纳米粒子相比,作用在具有超薄壳层厚度的 Au-Ag 核壳纳米粒子上的横向光扭矩可以增强两个数量级以上。这种增强的横向光扭矩主要由入射光场与偶极核壳纳米粒子中激发的电四极之间的相互作用决定。因此,需要注意的是,即使在偶极情况下,基于偶极子近似的扭矩表达式通常也不适用于偶极子粒子。这些发现加深了对光扭矩(OT)的物理理解,并可能在光驱动等离子体微粒子旋转方面具有应用。