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河流管理对美国不同河流中微塑料迁移的普遍影响:重新思考全球微塑料通量估算。

Prevailing impacts of river management on microplastic transport in contrasting US streams: Rethinking global microplastic flux estimations.

机构信息

School of Geography, Earth and Environmental Sciences, University of Birmingham, Edgbaston, Birmingham B15 2TT, United Kingdom.

U.S. Geological Survey, Colorado Water Science Center, 3215 Marine St, Boulder, Colorado 80303, United States.

出版信息

Water Res. 2023 Jul 15;240:120112. doi: 10.1016/j.watres.2023.120112. Epub 2023 May 24.

DOI:10.1016/j.watres.2023.120112
PMID:37257293
Abstract

While microplastic inputs into rivers are assumed to be correlated with anthropogenic activities and to accumulate towards the sea, the impacts of water management on downstream microplastic transport are largely unexplored. A comparative study of microplastic abundance in Boulder Creek (BC), and its less urbanized tributary South Boulder Creek (SBC), (Colorado USA), characterized the downstream evolution of microplastics in surface water and sediments, evaluating the effects of urbanization and flow diversions on the up-to-downstream profiles of microplastic concentrations and loads. Water and sediment samples were collected from 21 locations along both rivers and microplastic properties determined by fluorescence microscopy and Raman spectroscopy. The degree of catchment urbanization affected microplastic patterns, as evidenced by greater water and sediment concentrations and loads in BC than the less densely populated SBC, which is consistent with the differences in the degree of urbanization between both catchments. Microplastic removal through flow diversions was quantified, showing that water diversions removed over 500 microplastic particles per second from the river, and caused stepwise reductions of downstream loads at diversion points. This redistribution of microplastics back into the catchment should be considered in large scale models quantifying plastic fate and transport to the oceans.

摘要

尽管人们认为河流中的微塑料输入与人为活动有关,并向海洋聚集,但水管理对下游微塑料迁移的影响在很大程度上仍未得到探索。对美国科罗拉多州博尔德溪(BC)及其城市化程度较低的支流南博尔德溪(SBC)中的微塑料丰度进行了比较研究,该研究描述了地表水和沉积物中微塑料的下游演变,评估了城市化和水流分流对微塑料浓度和负荷的上下游分布的影响。从两条河流的 21 个地点采集了水和沉积物样本,并通过荧光显微镜和拉曼光谱法确定了微塑料的特性。集水区的城市化程度影响了微塑料的分布模式,这从 BC 比人口密度较低的 SBC 具有更高的水和沉积物浓度和负荷得到了证明,这与两个集水区之间的城市化程度差异是一致的。通过水流分流来去除微塑料的程度进行了量化,结果表明,水流分流每秒从河流中去除了超过 500 个微塑料颗粒,并在分流点造成了下游负荷的逐步减少。在将塑料命运和运输到海洋的大规模模型中,应该考虑这种将微塑料重新分配回集水区的情况。

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