School of Geography, Earth and Atmospheric Sciences, University of Melbourne, Melbourne, VIC, 3053, Australia.
The Peter Cook Centre for Carbon Capture and Storage Research, University of Melbourne, Melbourne, VIC, 3053, Australia.
Sci Rep. 2023 Jun 8;13(1):9334. doi: 10.1038/s41598-023-36349-0.
Carbon capture and storage is a key technology to abate CO emissions. One of the challenges towards ensuring the efficiency and the security of CO storage in reservoirs, such as open saline aquifers, is the low pore space utilization. This study investigates the feasibility of using an artificial Si-gel barrier to enhance pore space utilisation in such reservoirs under variable geological conditions. Conceptually, enhanced CO capillary trapping is achieved by emplacing a disk-shaped, low-permeability barrier above the CO injection point forcing the injected CO to migrate laterally underneath the barrier before transitioning to buoyancy-controlled migration. Multiphase fluid flow simulations were conducted to test the feasibility of this concept. Sensitivity analysis revealed that the barrier exhibits a strong control on CO plume geometry. Specifically, the relative impact of the barrier diameter on increasing the CO plume width, reducing the plume height and enhancing trapping varied between 67 and 86%. Capillary trapping was enhanced by 40-60% with a 20 m increase in barrier diameter in low permeability reservoirs. Additionally, the results indicate that the barrier can enhance the security of trapping CO in high permeability reservoirs. Results were tested for the South-West Hub reservoir, a case study area in Western Australia.
碳捕集与封存是减少 CO 排放的关键技术。在确保储层(如开放的盐含水层)中 CO 封存效率和安全性的诸多挑战中,一个挑战是孔隙空间利用率低。本研究探讨了在不同地质条件下,使用人工硅凝胶障壁来提高此类储层中孔隙空间利用率的可行性。从概念上讲,通过在 CO 注入点上方布置一个盘形低渗透率障壁,增强 CO 毛细捕获,迫使注入的 CO 在迁移到浮力控制迁移之前在障壁下方横向迁移。进行了多相流体流动模拟以测试该概念的可行性。敏感性分析表明,障壁对 CO 羽流几何形状具有很强的控制作用。具体而言,障壁直径对增加 CO 羽流宽度、降低羽流高度和增强捕获的相对影响在 67%至 86%之间变化。在低渗透率储层中,障壁直径增加 20 米可将毛细捕获提高 40-60%。此外,结果表明障壁可以提高高渗透率储层中 CO 捕获的安全性。结果针对西澳大利亚西南部枢纽储层进行了测试,这是一个案例研究区。