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磁场诱导的 Shastry-Sutherland 格子中的局域无序。

Field-induced partial disorder in a Shastry-Sutherland lattice.

机构信息

Neutron Scattering Division, Oak Ridge National Laboratory, Oak Ridge, TN, 37831, USA.

Department of Physics, University of Arizona, Tucson, AZ, 85721, USA.

出版信息

Nat Commun. 2023 Jun 19;14(1):3641. doi: 10.1038/s41467-023-39409-1.

Abstract

A 2-Q antiferromagnetic order of the ferromagnetic dimers was found below T = 2.9 K in the Shastry-Sutherland lattice BaNdZnS by single crystal neutron diffraction. The magnetic order can be understood by the orthogonal arrangement of local Ising Nd spins, identified by polarized neutrons. A field was applied along [1 -1 0] to probe the observed metamagnetic transition in the magnetization measurement. The field decouples two magnetic sublattices corresponding to the propagation vectors q = (½, ½, 0) and q = (-½, ½, 0), respectively. Each sublattice shows a "stripe" order with a Néel-type arrangement in each single layer. The "stripe" order with q remains nearly intact up to 6 T, while the other one with q is suppressed at a critical field H ~1.7 T, indicating a partial disorder. The H varies with temperature and is manifested in the H-T phase diagram constructed by measuring the magnetization in BaNdZnS.

摘要

通过单晶中子衍射发现,Shastry-Sutherland 晶格 BaNdZnS 在 T=2.9K 以下呈现出 2-Q 反铁磁有序。通过极化中子可以识别出局部 Ising Nd 自旋的正交排列,从而理解这种磁有序。磁场沿 [1-1-0] 方向施加,以探测磁化测量中观察到的顺磁转变。该磁场分别解耦了对应于传播矢量 q = (1/2, 1/2, 0) 和 q = (-1/2, 1/2, 0) 的两个磁子晶格。每个子晶格都呈现出具有尼尔型排列的“条纹”有序。具有 q 的“条纹”有序在高达 6T 的范围内几乎保持完整,而另一个具有 q 的有序则在临界场 H~1.7T 处被抑制,表明存在部分无序。H 随温度变化,并通过测量 BaNdZnS 中的磁化来构建 H-T 相图得以体现。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a4aa/10279730/5cb1f4de2395/41467_2023_39409_Fig1_HTML.jpg

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