Qin Zhengsheng, Wang Tianyu, Gao Haikuo, Li Yang, Dong Huanli, Hu Wenping
Beijing National Laboratory for Molecular Sciences, Key Laboratory of Organic Solids, Institute of Chemistry, Chinese Academy of Sciences, Beijing, 100190, China.
School of Chemical Sciences, University of Chinese Academy of Sciences, Beijing, 100049, China.
Adv Mater. 2023 Oct;35(40):e2301955. doi: 10.1002/adma.202301955. Epub 2023 Aug 7.
Electrically driven polarized light-emitting sources are central to various applications including quantum computers, optical communication, and 3D displays, but serious challenges remain due to the inevitable incorporation of complex optical elements in conventional devices. Here, organic polarized light-emitting transistors (OPLETs), a kind of novel device that integrates the functions of organic field-effect transistors, organic light-emitting diodes, and polarizers into one unique device, are demonstrated with a degree of polarization (DOP) as high as 0.97, which is comparable to completely linearly polarized light (DOP = 1). Under the modulation of gate voltage, robust and efficient polarization emission is proven, ascribed to the intrinsic in-plane anisotropy of the molecular transition dipole moment in organic semiconductors and the open-ended feature of OPLETs instead of other factors. As a result, high-contrast optical imaging and anti-counterfeiting security are successfully demonstrated based on OPLETs, establishing a new direction for photonic and electronic integration toward on-chip miniaturized optoelectronic applications.
电驱动的偏振发光源对于包括量子计算机、光通信和3D显示器在内的各种应用至关重要,但由于传统器件中不可避免地要集成复杂的光学元件,因此仍然面临严峻挑战。在此,展示了一种有机偏振发光晶体管(OPLETs),这是一种将有机场效应晶体管、有机发光二极管和偏振器的功能集成到一个独特器件中的新型器件,其偏振度(DOP)高达0.97,可与完全线偏振光(DOP = 1)相媲美。在栅极电压的调制下,证明了其具有稳健且高效的偏振发射,这归因于有机半导体中分子跃迁偶极矩的固有面内各向异性以及OPLETs的开放式结构,而非其他因素。结果,基于OPLETs成功展示了高对比度光学成像和防伪安全性,为实现片上小型化光电子应用的光子与电子集成开辟了新方向。