Institut de Química Computacional i Catàlisi and Departament de Química, Universitat de Girona, C/Maria Aurèlia Capmany, 69, 17003 Girona, Catalunya Spain.
Org Lett. 2023 Jul 7;25(26):4830-4834. doi: 10.1021/acs.orglett.3c01538. Epub 2023 Jun 26.
The selective assembly of the 1,4-oxathiin nucleus has been treated as a powerful strategy to access this scaffold present in molecules with very interesting properties. In this study, the chameleon-like reactivity of pyridinium 1,4-zwitterionic thiolates is exploited to assemble the 1,4-oxathiin core through a [3 + 3] annulation. The optimal annulation partner has been found to be the iodonium ylide of the cyclic 1,3-diketones. The developed protocol allows the synthesis of a variety of bicyclic 1,4-oxathiin derivatives under very mild conditions under copper(I) iodide catalysis. Access to benzoannulated 1,4-oxathiins has been achieved through iodine-mediated aromatization of the initially obtained bicyclic compounds.
1,4-氧硫杂环戊烷核的选择性组装已被视为一种强大的策略,可用于构建具有非常有趣性质的分子中存在的这种支架。在这项研究中,利用吡啶鎓 1,4-两性离子硫醇盐的变色龙般的反应性,通过[3 + 3]环加成来组装 1,4-氧硫杂环戊烷核心。已经发现最佳的环加成伙伴是环状 1,3-二酮的碘鎓叶立德。所开发的方案允许在碘化亚铜催化下,在非常温和的条件下,通过铜(I)碘化物合成各种双环 1,4-氧硫杂环戊烷衍生物。通过初始获得的双环化合物的碘介导芳构化,可以获得苯并稠合的 1,4-氧硫杂环戊烷。