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中国长三角太浦河两岸表土中多环芳烃:分布、来源及风险评估。

Polycyclic Aromatic Hydrocarbons in Topsoils Along the Taipu River Banks in the Yangtze River Delta, China: Occurrence, Source and Risk Assessment.

机构信息

School of Environmental and Geographical Sciences, Shanghai Normal University, Shanghai, 200234, China.

Yangtze River Delta Urban Wetland Ecosystem National Field Scientific Observation and Research Station, Shanghai, 201722, China.

出版信息

Bull Environ Contam Toxicol. 2023 Jun 26;111(1):9. doi: 10.1007/s00128-023-03751-3.

Abstract

Taipu River is an important transboundary river and drinking water source in the Yangtze River Delta, China. This study collected 15 topsoil samples along the Taipu River banks and subsequently determined the polycyclic aromatic hydrocarbons (PAHs) concentrations, sources, and ecological and health risks. The sum of toxic 15 PAHs concentrations ranged from 83.13 to 28342.53 ng/g, with a mean of 2828.69 ng/g. High molecular weight (HMW) PAHs were the dominant components and Indene (1,2,3, -cd) benzopyrene (InP) accounted for the highest proportion in individuals. The average PAH concentration in residential land was the highest, followed by those in industrial and agricultural land. The PAH concentration was positively related to contents of total carbon, total nitrogen, ammonium nitrogen, and aminopeptidase activity in soils. The mixed combustion of biomass, coal, and petroleum and traffic emissions could be the primary PAH contributors. The total PAHs at over half of sampling points had relatively high risk quotients and incremental lifetime cancer risk (ILCR) values, posing potential or great ecological threats and health risks.

摘要

太浦河是中国长江三角洲地区的一条重要跨界河流和饮用水源。本研究采集了太浦河两岸的 15 个表层土壤样本,随后测定了多环芳烃(PAHs)的浓度、来源、生态和健康风险。有毒 15 种多环芳烃的总浓度范围为 83.13 至 28342.53ng/g,平均值为 2828.69ng/g。高分子量(HMW)PAHs 是主要成分,茚并(1,2,3-cd)芘(InP)在个体中占比最高。住宅用地的 PAH 浓度最高,其次是工业和农业用地。PAH 浓度与土壤中总碳、总氮、氨氮和氨基肽酶活性的含量呈正相关。生物质、煤炭和石油的混合燃烧以及交通排放可能是 PAHs 的主要来源。超过一半采样点的总多环芳烃具有相对较高的风险商数和增量终生癌症风险(ILCR)值,对生态系统构成潜在或重大威胁,对人类健康也具有较高风险。

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