Xiao Yu-Xuan, Ying Jie, Liu Hong-Wei, Yang Xiao-Yu
School of Chemical Engineering and Technology, Sun Yat-sen University, Zhuhai, 519082 China.
State Key Laboratory of Advanced Technology for Materials Synthesis and Processing & Shenzhen Research Institute & Joint Laboratory for Marine Advanced Materials in Pilot National Laboratory for Marine Science and Technology (Qingdao), Wuhan University of Technology, Wuhan, 430070 China.
Front Chem Sci Eng. 2023 Apr 25:1-21. doi: 10.1007/s11705-023-2300-5.
Carbon-supported Pt-based materials are highly promising electrocatalysts. The carbon support plays an important role in the Pt-based catalysts by remarkably influencing the growth, particle size, morphology, dispersion, electronic structure, physiochemical property and function of Pt. This review summarizes recent progress made in the development of carbon-supported Pt-based catalysts, with special emphasis being given to how activity and stability enhancements are related to Pt-C interactions in various carbon supports, including porous carbon, heteroatom doped carbon, carbon-based binary support, and their corresponding electrocatalytic applications. Finally, the current challenges and future prospects in the development of carbon-supported Pt-based catalysts are discussed.
碳载铂基材料是极具前景的电催化剂。碳载体在铂基催化剂中起着重要作用,它能显著影响铂的生长、粒径、形态、分散性、电子结构、物理化学性质及功能。本文综述了碳载铂基催化剂开发方面的最新进展,特别强调了活性和稳定性的提高与各种碳载体(包括多孔碳、杂原子掺杂碳、碳基二元载体)中铂 - 碳相互作用的关系,以及它们相应的电催化应用。最后,讨论了碳载铂基催化剂开发中当前面临的挑战和未来前景。