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碳载铂基电催化剂中的铂-碳相互作用

Pt-C interactions in carbon-supported Pt-based electrocatalysts.

作者信息

Xiao Yu-Xuan, Ying Jie, Liu Hong-Wei, Yang Xiao-Yu

机构信息

School of Chemical Engineering and Technology, Sun Yat-sen University, Zhuhai, 519082 China.

State Key Laboratory of Advanced Technology for Materials Synthesis and Processing & Shenzhen Research Institute & Joint Laboratory for Marine Advanced Materials in Pilot National Laboratory for Marine Science and Technology (Qingdao), Wuhan University of Technology, Wuhan, 430070 China.

出版信息

Front Chem Sci Eng. 2023 Apr 25:1-21. doi: 10.1007/s11705-023-2300-5.

Abstract

Carbon-supported Pt-based materials are highly promising electrocatalysts. The carbon support plays an important role in the Pt-based catalysts by remarkably influencing the growth, particle size, morphology, dispersion, electronic structure, physiochemical property and function of Pt. This review summarizes recent progress made in the development of carbon-supported Pt-based catalysts, with special emphasis being given to how activity and stability enhancements are related to Pt-C interactions in various carbon supports, including porous carbon, heteroatom doped carbon, carbon-based binary support, and their corresponding electrocatalytic applications. Finally, the current challenges and future prospects in the development of carbon-supported Pt-based catalysts are discussed.

摘要

碳载铂基材料是极具前景的电催化剂。碳载体在铂基催化剂中起着重要作用,它能显著影响铂的生长、粒径、形态、分散性、电子结构、物理化学性质及功能。本文综述了碳载铂基催化剂开发方面的最新进展,特别强调了活性和稳定性的提高与各种碳载体(包括多孔碳、杂原子掺杂碳、碳基二元载体)中铂 - 碳相互作用的关系,以及它们相应的电催化应用。最后,讨论了碳载铂基催化剂开发中当前面临的挑战和未来前景。

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