Chen Yu, Yin Kai, Xu Yuxuan, Liu Min, Huang Han, Ouyang Fangping
School of Physics and Electronics and Institution of Super-Microstructure and Ultrafast Process in Advanced Materials, Central South University, 932 Lushannan Road, Changsha 410083, China.
Powder Metallurgy Research Institution and State Key Laboratory of Powder Metallurgy, Central South University, 932 Lushannan Road, Changsha 410083, China.
Nanomaterials (Basel). 2023 Jun 8;13(12):1826. doi: 10.3390/nano13121826.
The remote excitation and remote-controlling of the localized surface plasmon resonance (LSPR) in a heterotype and hollow gold nanosheet (HGNS) is studied using FDTD simulations. The heterotype HGNS contains an equilateral and hollow triangle in the center of a special hexagon, which forms a so-called hexagon-triangle (H-T) heterotype HGNS. If we focus the incident-exciting laser on one of the vertexes of the center triangle, the LSPR could be achieved among other remote vertexes of the outer hexagon. The LSPR wavelength and peak intensity depend sensitively on factors such as the polarization of the incident light, the size and symmetry of the H-T heterotype structure, etc. Several groups of the optimized parameters were screened out from numerous FDTD calculations, which help to further obtain some significant polar plots of the polarization-dependent LSPR peak intensity with two-petal, four-petal or six-petal patterns. Remarkably, based on these polar plots, the on-off switching of the LSPR coupled among four HGNS hotspots could be remote-controlled simply via only one polarized light, which shows promise for its potential application in remote-controllable surface-enhanced Raman scattering (SERS), optical interconnects and multi-channel waveguide switches.
利用时域有限差分(FDTD)模拟研究了异型中空金纳米片(HGNS)中局域表面等离子体共振(LSPR)的远程激发和远程控制。异型HGNS在一个特殊六边形的中心包含一个等边中空三角形,形成了所谓的六边形 - 三角形(H - T)异型HGNS。如果将入射激发激光聚焦在中心三角形的一个顶点上,那么在外六边形的其他远程顶点之间就可以实现LSPR。LSPR波长和峰值强度敏感地取决于诸如入射光的偏振、H - T异型结构的尺寸和对称性等因素。从大量的FDTD计算中筛选出了几组优化参数,这有助于进一步获得一些具有两瓣、四瓣或六瓣图案的与偏振相关的LSPR峰值强度的重要极坐标图。值得注意的是,基于这些极坐标图,仅通过一束偏振光就可以远程控制四个HGNS热点之间耦合的LSPR的开 - 关切换,这显示了其在远程可控表面增强拉曼散射(SERS)、光互连和多通道波导开关中的潜在应用前景。