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明渠水流中遮蔽物对微塑料迁移影响的研究

Investigation of the Sheltering Effects on the Mobilization of Microplastics in Open-Channel Flow.

作者信息

Yu Zijian, Loewen Mark, Guo Shuai, Guo Zhiyong, Zhang Wenming

机构信息

Department of Civil and Environmental Engineering, University of Alberta, Edmonton, AB, Canada T6G 1H9.

Department of Municipal Engineering, Hefei University of Technology, Hefei 230009, China.

出版信息

Environ Sci Technol. 2023 Aug 1;57(30):11259-11266. doi: 10.1021/acs.est.3c02500. Epub 2023 Jul 20.

Abstract

Microplastics (MPs) can be sheltered by bed grains, resulting in a higher threshold of mobilization compared with those moving on a smooth bed. Only one formula considering the sheltering effects has been proposed for the critical shear stress () of MP mobilization by including the densities and sizes of MPs and bed grains, but it is inaccurate for MPs of certain materials such as PS and shows limitations in understanding the sheltering effects. Additionally, no method exists for the critical depth-averaged velocity (). In this study, experiments were conducted measuring both and of MPs (made of PA, PVC, and PET) deposited on rough beds of different roughnesses, with a focus on the sheltering effects. A power law relationship between and the density and size of MPs was found, and a new formula for estimating was proposed for MPs, which reduced the errors by approximately 40% compared with that of the previous formula (27.8%). To explicitly quantify the sheltering effects in MP mobilizations, hiddenness (), exposure (), and longitudinal exposure () were introduced, all of which were observed to follow a normal distribution. A semiempirical method for was then proposed incorporating the new measures, which reduced the errors by around 70% compared to the methods developed for estimating the values of sediments.

摘要

微塑料(MPs)可被床沙颗粒遮蔽,与在光滑床面上移动的微塑料相比,其启动阈值更高。仅提出了一个考虑遮蔽效应的公式,用于计算微塑料启动的临界剪应力(),该公式纳入了微塑料和床沙颗粒的密度及尺寸,但对于某些材料(如聚苯乙烯)的微塑料并不准确,且在理解遮蔽效应方面存在局限性。此外,尚无计算临界深度平均流速()的方法。在本研究中,进行了实验,测量了沉积在不同粗糙度粗糙床面上的微塑料(由聚酰胺、聚氯乙烯和聚对苯二甲酸乙二酯制成)的和,重点关注遮蔽效应。发现了与微塑料密度和尺寸之间的幂律关系,并提出了一个估算微塑料的新公式,与先前公式相比,该公式的误差降低了约40%(27.8%)。为明确量化微塑料启动中的遮蔽效应,引入了隐蔽度()、暴露度()和纵向暴露度(),观察发现它们均服从正态分布。然后提出了一种结合新测量值的半经验方法来计算,与用于估算沉积物值的方法相比,该方法的误差降低了约70%。

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