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嵌入微腔中的离散溴化铯铅量子点实现稳定连续波激光发射。

Stable continuous-wave lasing from discrete cesium lead bromide quantum dots embedded in a microcavity.

作者信息

Zhang Hongbo, Wen Wen, Du Bowen, Zhou Lei, Chen Yu, Feng Shun, Zou Chenji, Wu Lishu, Fan Hong Jin, Gao Weibo, Sun Handong, Shang Jingzhi, Yu Ting

机构信息

Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University, Singapore 637371, Singapore.

College of Physics and Optoelectronic Engineering, Shenzhen University, Shenzhen 518060, China.

出版信息

Nanoscale Horiz. 2023 Sep 26;8(10):1403-1410. doi: 10.1039/d3nh00139c.

Abstract

All-inorganic cesium lead bromide (CsPbBr) quantum dots (QDs) with high photoluminescence (PL) quantum efficiency have been reported as ideal gain materials for high-performance lasers. Nevertheless, isolated CsPbBr QDs have not achieved lasing emission (LE) due to finite absorption cross-section. Here, we demonstrate continuous-wave lasing of isolated CsPbBr QDs embedded in a microcavity. Distributed Bragg reflectors (DBRs), together with isolated CsPbBr QDs in a polymer matrix, are introduced to construct a vertical-cavity surface-emitting laser (VCSEL), which exhibits stable single-mode lasing emissions with an ultra-low threshold of 8.8 W cm and a high factor of 1787. Such perovskite-based microcavity structures sustain highly stable excitons at room temperature and can provide an excellent experimental platform to further study the single-particle nano-lasers and quantum physics frontiers such as exciton-polariton condensation, single-photon emission, and optical quantum communication.

摘要

具有高光致发光(PL)量子效率的全无机铯铅溴化物(CsPbBr)量子点(QDs)已被报道为高性能激光器的理想增益材料。然而,由于有限的吸收截面,孤立的CsPbBr量子点尚未实现激光发射(LE)。在此,我们展示了嵌入微腔中的孤立CsPbBr量子点的连续波激光发射。引入分布式布拉格反射器(DBR)以及聚合物基质中的孤立CsPbBr量子点,以构建垂直腔面发射激光器(VCSEL),该激光器表现出稳定的单模激光发射,超低阈值为8.8 W/cm²,品质因数高达1787。这种基于钙钛矿的微腔结构在室温下维持高度稳定的激子,并可为进一步研究单粒子纳米激光器和量子物理前沿(如激子极化激元凝聚、单光子发射和光量子通信)提供出色的实验平台。

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