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多色碳点的合成策略、性质及传感应用:最新进展与未来挑战。

Synthetic strategies, properties and sensing application of multicolor carbon dots: recent advances and future challenges.

机构信息

Postdoctoral Research Station of Basic Medicine, School of Pharmaceutical Science, Hengyang Medical School, University of South China, Hengyang, Hunan, 421001, China.

出版信息

J Mater Chem B. 2023 Aug 30;11(34):8117-8135. doi: 10.1039/d3tb01329d.

Abstract

Recently, carbon dots (CDs) as newly developed carbon-based nanomaterials due to advantages such as excellent photostability and easy surface functionalization have generated wide application prospects in fields such as biological imaging and chemical sensing. The multicolor emission carbon dots (M-CDs) were acquired through the selection of different carbon source precursors, change of synthesis conditions and synthesis environment. Therefore, the aim of this review is to summarize the latest research progress in polychromatic CDs from the perspectives of synthesis strategies, luminescent mechanisms, luminescent properties and applications. This review focuses on how to prepare MCDs by changing raw materials and synthesis conditions such as reaction temperature, synthesis time, synthesis pH, and synthesis solvent. This review also presents the optical properties of MCDs, concentration effects, solvent effects, pH effects, elemental doping, and surface passivation on them, as well as their creative applications in the field of sensing applications. It is anticipated that this review will serve as a guide for the development of multifunctional M-CDs and inspire future research on controllable design and preparation of M-CDs.

摘要

最近,由于具有优异的光稳定性和易于表面功能化等优点,碳点(CDs)作为新型碳基纳米材料,在生物成像和化学传感等领域产生了广泛的应用前景。多色发射碳点(M-CDs)是通过选择不同的碳源前体、改变合成条件和合成环境获得的。因此,本综述的目的是从合成策略、发光机制、发光性能和应用等方面总结多色碳点的最新研究进展。本综述重点介绍了如何通过改变反应温度、合成时间、合成 pH 值和合成溶剂等合成条件以及原料来制备 MCDs。本综述还介绍了 MCDs 的光学性质、浓度效应、溶剂效应、pH 值效应、元素掺杂和表面钝化及其在传感应用领域的创造性应用。预计本综述将为多功能 M-CDs 的开发提供指导,并激发对 M-CDs 的可控设计和制备的未来研究。

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