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银纳米颗粒诱导二维发光二极管中光提取的增强。

Silver nanoparticle-induced enhancement of light extraction in two-dimensional light-emitting diodes.

作者信息

Liu Tianqi, Fu Qiang, Li Yuanzhe, Han Xu, Wang Shixuan, Taniguchi Takashi, Watanabe Kenji, Wan Dongyang, Zhang Qi, Zhao Yingbo, Ni Zhenhua, Ding Fei, Hu Zhenliang, Yuan Xueyong, Lu Junpeng

出版信息

Opt Lett. 2023 Aug 15;48(16):4372-4375. doi: 10.1364/OL.498850.

Abstract

Monolayer transition metal dichalcogenides (TMDCs) with direct bandgaps are considered promising candidates for building light-emitting diodes (LEDs). One crucial indicator of their performance is the brightness of electroluminescence (EL). In this study, we fabricate WS-based LEDs that make full use of the assistance of effective transient-mode charge injection. By introducing self-assembled silver nanoparticles (NPs) on top of the LED, the extraction efficiency is significantly improved, with a 2.9-fold EL enhancement observed in the experiment. Full-wave simulations further confirm that the improvement comes from the scattering capability of silver NPs, with results qualitatively fitting the experiment. This approach, with its compatibility with van der Waals heterostructures, can be further promoted to enhance the brightness of 2D monolayer TMDC-based LEDs.

摘要

具有直接带隙的单层过渡金属二硫属化物(TMDCs)被认为是制造发光二极管(LEDs)的有前途的候选材料。其性能的一个关键指标是电致发光(EL)的亮度。在本研究中,我们制造了基于WS的LED,充分利用了有效瞬态模式电荷注入的辅助作用。通过在LED顶部引入自组装银纳米颗粒(NPs),提取效率显著提高,实验中观察到EL增强了2.9倍。全波模拟进一步证实,这种改善来自银纳米颗粒的散射能力,结果在定性上与实验相符。这种方法与范德华异质结构兼容,可以进一步推广以提高基于二维单层TMDC的LED的亮度。

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