Hu Gongwei, Huang Fobao, Liu Jun-Feng
School of Physics and Materials Science, Guangzhou University, Guangzhou 510006, China.
School of Microelectronics, Northwestern Polytechnical University, Xi'an 710072, China.
Phys Chem Chem Phys. 2023 Aug 30;25(34):23001-23011. doi: 10.1039/d3cp02902f.
The combination of piezoelectricity and spin-orbit coupling (SOC) effect makes wurtzite semiconductors attractive for the development of exotic spin-related physics as well as spintronic applications. Triggering piezoelectricity, particularly by an external stimulus, provides a new perspective for manipulating SOC, but until now, a comprehensive understanding of this mechanism is lacking. Herein, by means of self-consistent calculations and Löwdin perturbation approach, we have explored the manipulation of SOC in the wurtzite (Al, Ga)N/GaN heterostructure by external stress-induced piezoelectric polarization. The results suggest that the Rashba SOC depends weakly on stress due to the wide-gap feature of the wurtzite crystal that makes Rashba SOC predominant by a bulk term instead of the structural inversion term. The piezoelectric polarization diminishes and even turns off Dresselhaus coupling by reducing the interfacial electric field. Moreover, piezoelectricity is shown to improve the poorly gate-tunable SOC. In the heterostructure with two occupied subbands, the Dresselhaus coupling of the second subband is more sensitive than the first one in response to stress. As an extension, we further demonstrate that the correlation effect in the wurtzite heterostructure can be significantly enhanced by piezoelectric polarization. This study offers an in-depth insight into piezoelectric modulation of spin-orbit physics, which has the potential for stimulating new quantum correlation states or designing functional spintronic devices.
压电性与自旋轨道耦合(SOC)效应的结合,使得纤锌矿半导体在奇异的自旋相关物理以及自旋电子学应用的发展方面具有吸引力。触发压电性,特别是通过外部刺激来触发,为操纵SOC提供了一个新的视角,但到目前为止,对这种机制还缺乏全面的理解。在此,通过自洽计算和洛丁微扰方法,我们研究了外部应力诱导的压电极化对纤锌矿(Al,Ga)N/GaN异质结构中SOC的操纵。结果表明,由于纤锌矿晶体的宽带隙特性,使得Rashba SOC主要由体项而非结构反演项主导,因此Rashba SOC对应力的依赖较弱。压电极化通过降低界面电场来减弱甚至消除Dresselhaus耦合。此外,可以证明压电性能够改善栅极可调性较差的SOC。在具有两个占据子带的异质结构中,第二个子带的Dresselhaus耦合对应力的响应比第一个子带更敏感。作为一种拓展,我们进一步证明了纤锌矿异质结构中的关联效应可以通过压电极化得到显著增强。这项研究为自旋轨道物理的压电调制提供了深入的见解,具有激发新的量子关联态或设计功能性自旋电子器件的潜力。