Dipartimento di Chimica, Università degli Studi di Bari Aldo Moro, via Orabona 4, 70126, Bari, Italy.
Dipartimento di Bioscienze, Biotecnologie e Ambiente, Università degli Studi di Bari Aldo Moro, via Orabona 4, 70126, Bari, Italy.
Sci Rep. 2023 Aug 26;13(1):13972. doi: 10.1038/s41598-023-40357-5.
The occurrence of methyl carbamates of phosphatidylethanolamines and phosphatidylserines in the lipid extract of mitochondria obtained from mouse embryonic fibroblasts was ascertained by hydrophilic interaction liquid chromatography with electrospray ionization single and multi-stage mass spectrometry, performed using sinergically a high resolution (quadrupole-Orbitrap) and a low resolution (linear ion trap) spectrometer. Two possible routes to the synthesis of methyl carbamates of phospholipids were postulated and evaluated: (i) a chemical transformation involving phosgene, occurring as a photooxidation by-product in the chloroform used for lipid extraction, and methanol, also used for the latter; (ii) an enzymatic methoxycarbonylation reaction due to an accidental bacterial contamination, that was unveiled subsequently on the murine mitochondrial sample. A specific lipid extraction performed on a couple of standard phosphatidyl-ethanolamines/-serines, based on purposely photo-oxidized chloroform and deuterated methanol, indicated route (i) as negligible in the specific case, thus highlighting the enzymatic route related to bacterial contamination as the most likely source of methyl carbamates. The unambiguous recognition of the latter might represent the starting point toward a better understanding of their generation in biological systems and a minimization of their occurrence when an artefactual formation is ascertained.
通过亲水相互作用液相色谱-电喷雾电离单级和多级质谱法,使用高分辨率(四极杆-Orbitrap)和低分辨率(线性离子阱)质谱仪协同作用,确定了从小鼠胚胎成纤维细胞线粒体脂质提取物中获得的磷脂乙醇胺和磷脂酰丝氨酸的甲基氨基甲酸酯的存在。提出并评估了合成磷脂甲基氨基甲酸酯的两种可能途径:(i)涉及光气的化学转化,作为用于脂质提取的氯仿中的光氧化副产物,以及甲醇,也用于后者;(ii)由于偶然的细菌污染而发生的酶促甲氧基羰基化反应,随后在鼠线粒体样品中揭示了这种反应。在一对标准的磷脂乙醇胺/-丝氨酸上进行的特定脂质提取,基于故意光氧化的氯仿和氘化甲醇,表明在特定情况下途径 (i) 可以忽略不计,因此,与细菌污染相关的酶促途径是甲基氨基甲酸酯最可能的来源。后者的明确识别可能代表着更好地理解它们在生物系统中的生成以及在确定人为形成时减少其发生的起点。