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钨、钽和锇原子核的(n,2n)截面计算

(n,2n) cross section calculations for tungsten, tantalum and osmium nuclei.

作者信息

Yiğit Mustafa

机构信息

Department of Physics, Aksaray University, Aksaray, 68100, Turkey.

出版信息

Appl Radiat Isot. 2023 Nov;201:110999. doi: 10.1016/j.apradiso.2023.110999. Epub 2023 Aug 23.

Abstract

Tungsten, tantalum and osmium are important alloying elements in the nuclear technology research and development, particularly in nuclear fission/fusion power plant material applications. So, data results of the cross sections and emission spectra of neutron-induced reactions are required to predict nuclear responses in these elements. However, the cross sections measurements of (n,2n) reactions on tungsten, tantalum and osmium isotopes are rather limited in the literature. In this case, theoretical approaches are often used for obtaining the cross section data. In this article, theoretical (n,2n) cross sections on W, Ta and Os target nuclei are calculated up to 20 MeV energy, using the simulation codes TALYS 1.95, ALICE/ASH and CEM03.01. Further, the empirical (n,2n) systematics based on the statistical model have been used for predicting the cross section data at ∼14 MeV incident neutrons. The present results from the empirical systematics and model-based calculations are also compared with the literature experimental data, and JENDL-5.0, ENDF/B-VIII, JEFF3.3 and TENDL-2021 libraries. This paper can provide a contribution to complete description of the (n,2n) reactions considering the lack of experimental cross section data.

摘要

钨、钽和锇是核技术研发中的重要合金元素,尤其在核裂变/聚变发电厂材料应用方面。因此,需要中子诱发反应的截面和发射光谱数据结果来预测这些元素中的核反应。然而,文献中关于钨、钽和锇同位素的(n,2n)反应截面测量相当有限。在这种情况下,理论方法常被用于获取截面数据。在本文中,使用模拟代码TALYS 1.95、ALICE/ASH和CEM03.01计算了W、Ta和Os靶核上高达20 MeV能量的理论(n,2n)截面。此外,基于统计模型的经验(n,2n)系统atics已被用于预测约14 MeV入射中子时的截面数据。还将经验系统atics和基于模型计算的当前结果与文献实验数据以及JENDL - 5.0、ENDF/B - VIII、JEFF3.3和TENDL - 2021库进行了比较。考虑到缺乏实验截面数据,本文可为完整描述(n,2n)反应做出贡献。

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